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Main Authors: Meisenheimer, Peter, Moore, Guy, Zhou, Shiyu, Zhang, Hongrui, Huang, Xiaoxi, Husain, Sajid, Chen, Xianzhe, Martin, Lane W., Persson, Kristin A., Griffin, Sinéad, Caretta, Lucas, Stevenson, Paul, Ramesh, Ramamoorthy
Format: Preprint
Published: 2023
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Online Access:https://arxiv.org/abs/2311.10169
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author Meisenheimer, Peter
Moore, Guy
Zhou, Shiyu
Zhang, Hongrui
Huang, Xiaoxi
Husain, Sajid
Chen, Xianzhe
Martin, Lane W.
Persson, Kristin A.
Griffin, Sinéad
Caretta, Lucas
Stevenson, Paul
Ramesh, Ramamoorthy
author_facet Meisenheimer, Peter
Moore, Guy
Zhou, Shiyu
Zhang, Hongrui
Huang, Xiaoxi
Husain, Sajid
Chen, Xianzhe
Martin, Lane W.
Persson, Kristin A.
Griffin, Sinéad
Caretta, Lucas
Stevenson, Paul
Ramesh, Ramamoorthy
contents A key challenge in antiferromagnetic spintronics is the control of spin configuration on nanometer scales applicable to solid-state technologies. Bismuth ferrite (BiFeO3) is a multiferroic material that exhibits both ferroelectricity and canted antiferromagnetism at room temperature, making it a unique candidate in the development of electric-field controllable magnetic devices. The magnetic moments in BiFeO3 are arranged into a spin cycloid, resulting in unique magnetic properties which are tied to the ferroelectric order. Previous understanding of this coupling has relied on average, mesoscale measurements to infer behavior. Using nitrogen vacancy-based diamond magnetometry, we show that the spin cycloid can be deterministically controlled with an electric field. The energy landscape of the cycloid is shaped by both the ferroelectric degree of freedom and strain-induced anisotropy, restricting the magnetization changes to specific ferroelectric switching events. This study provides understanding of the antiferromagnetic texture in BiFeO3 and paves new avenues for designing magnetic textures and spintronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2311_10169
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Persistent anisotropy of the spin cycloid in BiFeO3 through ferroelectric switching
Meisenheimer, Peter
Moore, Guy
Zhou, Shiyu
Zhang, Hongrui
Huang, Xiaoxi
Husain, Sajid
Chen, Xianzhe
Martin, Lane W.
Persson, Kristin A.
Griffin, Sinéad
Caretta, Lucas
Stevenson, Paul
Ramesh, Ramamoorthy
Materials Science
A key challenge in antiferromagnetic spintronics is the control of spin configuration on nanometer scales applicable to solid-state technologies. Bismuth ferrite (BiFeO3) is a multiferroic material that exhibits both ferroelectricity and canted antiferromagnetism at room temperature, making it a unique candidate in the development of electric-field controllable magnetic devices. The magnetic moments in BiFeO3 are arranged into a spin cycloid, resulting in unique magnetic properties which are tied to the ferroelectric order. Previous understanding of this coupling has relied on average, mesoscale measurements to infer behavior. Using nitrogen vacancy-based diamond magnetometry, we show that the spin cycloid can be deterministically controlled with an electric field. The energy landscape of the cycloid is shaped by both the ferroelectric degree of freedom and strain-induced anisotropy, restricting the magnetization changes to specific ferroelectric switching events. This study provides understanding of the antiferromagnetic texture in BiFeO3 and paves new avenues for designing magnetic textures and spintronic devices.
title Persistent anisotropy of the spin cycloid in BiFeO3 through ferroelectric switching
topic Materials Science
url https://arxiv.org/abs/2311.10169