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Hauptverfasser: Manzhos, Sergei, Ihara, Manabu
Format: Preprint
Veröffentlicht: 2023
Schlagworte:
Online-Zugang:https://arxiv.org/abs/2311.10790
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author Manzhos, Sergei
Ihara, Manabu
author_facet Manzhos, Sergei
Ihara, Manabu
contents Kernel methods such as kernel ridge regression and Gaussian process regressions with Matern type kernels have been increasingly used, in particular, to fit potential energy surfaces (PES) and density functionals, and for materials informatics. When the dimensionality of the feature space is high, these methods are used with necessarily sparse data. In this regime, the optimal length parameter of a Matern-type kernel tends to become so large that the method effectively degenerates into a low-order polynomial regression and therefore loses any advantage over such regression. This is demonstrated theoretically as well as numerically on the examples of six- and fifteen-dimensional molecular PES using squared exponential and simple exponential kernels. The results shed additional light on the success of polynomial approximations such as PIP for medium size molecules and on the importance of orders-of-coupling based models for preserving the advantages of kernel methods with Matern type kernels or on the use of physically-motivated (reproducing) kernels.
format Preprint
id arxiv_https___arxiv_org_abs_2311_10790
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Degeneration of kernel regression with Matern kernels into low-order polynomial regression in high dimension
Manzhos, Sergei
Ihara, Manabu
Computational Physics
Machine Learning
Kernel methods such as kernel ridge regression and Gaussian process regressions with Matern type kernels have been increasingly used, in particular, to fit potential energy surfaces (PES) and density functionals, and for materials informatics. When the dimensionality of the feature space is high, these methods are used with necessarily sparse data. In this regime, the optimal length parameter of a Matern-type kernel tends to become so large that the method effectively degenerates into a low-order polynomial regression and therefore loses any advantage over such regression. This is demonstrated theoretically as well as numerically on the examples of six- and fifteen-dimensional molecular PES using squared exponential and simple exponential kernels. The results shed additional light on the success of polynomial approximations such as PIP for medium size molecules and on the importance of orders-of-coupling based models for preserving the advantages of kernel methods with Matern type kernels or on the use of physically-motivated (reproducing) kernels.
title Degeneration of kernel regression with Matern kernels into low-order polynomial regression in high dimension
topic Computational Physics
Machine Learning
url https://arxiv.org/abs/2311.10790