Magnetic-field-induced critical dynamics in magnetoelectric TbPO$_4$

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Hauptverfasser: Grams, Christoph P., Grüninger, Markus, Hemberger, Joachim
Format: Preprint
Veröffentlicht: 2023
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author Grams, Christoph P.
Grüninger, Markus
Hemberger, Joachim
author_facet Grams, Christoph P.
Grüninger, Markus
Hemberger, Joachim
contents We report on the magnetoelectric dynamics in the linear magnetoelectric antiferromagnet TbPO$_4$ studied by broadband dielectric spectroscopy. For the phase transition into the magnetoelectric antiferromagnetic phase at $T_{N} \approx 2.3$ K, a finite magnetic field $H$ induces critical behavior in the quasi-static permittivity $\varepsilon'$. Plotting the corresponding anomaly as function of $T/T_N(H)$, we observe the scaling behavior $Δ\varepsilon' \propto H^2$, a clear fingerprint of linear magnetoelectric antiferromagnets. Above the phase transition, we find a critical slowing down of the ferroic fluctuations in finite magnetic field. This behaviour can be understood via a magnetic-field-induced relaxational response that resembles the soft-mode behaviour in canonical ferroelectrics and multiferroics.
format Preprint
id arxiv_https___arxiv_org_abs_2312_00726
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Magnetic-field-induced critical dynamics in magnetoelectric TbPO$_4$
Grams, Christoph P.
Grüninger, Markus
Hemberger, Joachim
Strongly Correlated Electrons
We report on the magnetoelectric dynamics in the linear magnetoelectric antiferromagnet TbPO$_4$ studied by broadband dielectric spectroscopy. For the phase transition into the magnetoelectric antiferromagnetic phase at $T_{N} \approx 2.3$ K, a finite magnetic field $H$ induces critical behavior in the quasi-static permittivity $\varepsilon'$. Plotting the corresponding anomaly as function of $T/T_N(H)$, we observe the scaling behavior $Δ\varepsilon' \propto H^2$, a clear fingerprint of linear magnetoelectric antiferromagnets. Above the phase transition, we find a critical slowing down of the ferroic fluctuations in finite magnetic field. This behaviour can be understood via a magnetic-field-induced relaxational response that resembles the soft-mode behaviour in canonical ferroelectrics and multiferroics.
title Magnetic-field-induced critical dynamics in magnetoelectric TbPO$_4$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2312.00726