Extreme orbital ab-plane upper critical fields far beyond Pauli limit in 4Hb-Ta(S, Se)2 bulk crystals

Fuente: arXiv
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Autores principales: Meng, Fanyu, Fu, Yang, Pan, Senyang, Tian, Shangjie, Yan, Shaohua, Li, Zhengyu, Wang, Shouguo, Zhang, Jinglei, Lei, Hechang
Formato: Preprint
Publicado: 2023
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author Meng, Fanyu
Fu, Yang
Pan, Senyang
Tian, Shangjie
Yan, Shaohua
Li, Zhengyu
Wang, Shouguo
Zhang, Jinglei
Lei, Hechang
author_facet Meng, Fanyu
Fu, Yang
Pan, Senyang
Tian, Shangjie
Yan, Shaohua
Li, Zhengyu
Wang, Shouguo
Zhang, Jinglei
Lei, Hechang
contents Transition metal disulfides 4Hb-Ta(S, Se)2 with natural heterostructure of 1T- and 1H-Ta(S, Se)2 layers have became the focus of correlated materials their unique combinations of Mott physics and possible topological superconductivity. In this work, we study the upper critical fields mu0Hc2 of 4Hb-TaS2 and 4Hb-TaS1.99Se0.01 single crystals systematically. Transport measurements up to 35 T show that both of ab-plane and c-axis upper critical fields (mu0Hc2,ab and mu0Hc2,c) for 4Hb-TaS2 and 4Hb-TaS1.99Se0.01 exhibit a linear temperature dependent behavior down to 0.3 K, suggesting the three-dimensional superconductivity with dominant orbital depairing mechanism in bulk 4Hb-Ta(S, Se)2. However, the zero-temperature mu0Hc2,ab(0) for both crystals are far beyond the Pauli paramagnetic limit mu0HP. It could be explained by the effects of spin-momentum locking in 1H-Ta(S, Se)2 layers with local inversion symmetry broken and the relatively weak intersublattice interaction between 1H layers due to the existence of 1T layers.
format Preprint
id arxiv_https___arxiv_org_abs_2312_03448
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Extreme orbital ab-plane upper critical fields far beyond Pauli limit in 4Hb-Ta(S, Se)2 bulk crystals
Meng, Fanyu
Fu, Yang
Pan, Senyang
Tian, Shangjie
Yan, Shaohua
Li, Zhengyu
Wang, Shouguo
Zhang, Jinglei
Lei, Hechang
Superconductivity
Strongly Correlated Electrons
Transition metal disulfides 4Hb-Ta(S, Se)2 with natural heterostructure of 1T- and 1H-Ta(S, Se)2 layers have became the focus of correlated materials their unique combinations of Mott physics and possible topological superconductivity. In this work, we study the upper critical fields mu0Hc2 of 4Hb-TaS2 and 4Hb-TaS1.99Se0.01 single crystals systematically. Transport measurements up to 35 T show that both of ab-plane and c-axis upper critical fields (mu0Hc2,ab and mu0Hc2,c) for 4Hb-TaS2 and 4Hb-TaS1.99Se0.01 exhibit a linear temperature dependent behavior down to 0.3 K, suggesting the three-dimensional superconductivity with dominant orbital depairing mechanism in bulk 4Hb-Ta(S, Se)2. However, the zero-temperature mu0Hc2,ab(0) for both crystals are far beyond the Pauli paramagnetic limit mu0HP. It could be explained by the effects of spin-momentum locking in 1H-Ta(S, Se)2 layers with local inversion symmetry broken and the relatively weak intersublattice interaction between 1H layers due to the existence of 1T layers.
title Extreme orbital ab-plane upper critical fields far beyond Pauli limit in 4Hb-Ta(S, Se)2 bulk crystals
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2312.03448