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Main Authors: Hartman, Elrina, Tobar, Michael E, McAllister, Ben T, Bourhill, Jeremy, Goryachev, Maxim
Format: Preprint
Published: 2023
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Online Access:https://arxiv.org/abs/2312.05199
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author Hartman, Elrina
Tobar, Michael E
McAllister, Ben T
Bourhill, Jeremy
Goryachev, Maxim
author_facet Hartman, Elrina
Tobar, Michael E
McAllister, Ben T
Bourhill, Jeremy
Goryachev, Maxim
contents We present experimental observations of dilute ion spin ensemble defects in a low-loss single crystal cylindrical sample of CaWO$_4$ cooled to $30$ mK in temperature. Crystal field perturbations were elucidated by constructing a dielectrically loaded microwave cavity resonator from the crystal. The resonator exhibited numerous whispering gallery modes with high $Q$-factors of up to $3\times 10^7$, equivalent to a loss tangent of $\sim 3\times 10^{-8}$. The low loss allowed precision multi-mode spectroscopy of numerous high $Q$-factor photon-spin interactions. Measurements between 7 to 22 GHz revealed the presence of Gd$^{3+}$, Fe$^{3+}$, and another trace species, inferred to be rare-earth, at concentrations on the order of parts per billion. These findings motivate further exploration of prospective uses of this low-loss dielectric material for applications regarding precision and quantum metrology, as well as tests for beyond standard model physics.
format Preprint
id arxiv_https___arxiv_org_abs_2312_05199
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Precision Multi-Mode Microwave Spectroscopy of Paramagnetic and Rare-Earth Ion Spin Defects in Single Crystal Calcium Tungstate
Hartman, Elrina
Tobar, Michael E
McAllister, Ben T
Bourhill, Jeremy
Goryachev, Maxim
Quantum Physics
Materials Science
We present experimental observations of dilute ion spin ensemble defects in a low-loss single crystal cylindrical sample of CaWO$_4$ cooled to $30$ mK in temperature. Crystal field perturbations were elucidated by constructing a dielectrically loaded microwave cavity resonator from the crystal. The resonator exhibited numerous whispering gallery modes with high $Q$-factors of up to $3\times 10^7$, equivalent to a loss tangent of $\sim 3\times 10^{-8}$. The low loss allowed precision multi-mode spectroscopy of numerous high $Q$-factor photon-spin interactions. Measurements between 7 to 22 GHz revealed the presence of Gd$^{3+}$, Fe$^{3+}$, and another trace species, inferred to be rare-earth, at concentrations on the order of parts per billion. These findings motivate further exploration of prospective uses of this low-loss dielectric material for applications regarding precision and quantum metrology, as well as tests for beyond standard model physics.
title Precision Multi-Mode Microwave Spectroscopy of Paramagnetic and Rare-Earth Ion Spin Defects in Single Crystal Calcium Tungstate
topic Quantum Physics
Materials Science
url https://arxiv.org/abs/2312.05199