Biorealistic Response in Optoelectrically-Driven Flexible Halide-Perovskite Single-Crystal Memristors

Fuente: arXiv
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Autores principales: Matchenya, Ivan, Khanas, Anton, Podgornyi, Roman, Shirkin, Daniil, Ekgardt, Alexey, Sizykh, Nikita, Anoshkin, Sergey, Krasnikov, Dmitry V., Yulin, Alexei, Zhukov, Alexey, Nasibulin, Albert G., Scheblykin, Ivan, Pushkarev, Anatoly, Zenkevich, Andrei, Bisquert, Juan, Marunchenko, Alexandr
Formato: Preprint
Publicado: 2023
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author Matchenya, Ivan
Khanas, Anton
Podgornyi, Roman
Shirkin, Daniil
Ekgardt, Alexey
Sizykh, Nikita
Anoshkin, Sergey
Krasnikov, Dmitry V.
Yulin, Alexei
Zhukov, Alexey
Nasibulin, Albert G.
Scheblykin, Ivan
Pushkarev, Anatoly
Zenkevich, Andrei
Bisquert, Juan
Marunchenko, Alexandr
author_facet Matchenya, Ivan
Khanas, Anton
Podgornyi, Roman
Shirkin, Daniil
Ekgardt, Alexey
Sizykh, Nikita
Anoshkin, Sergey
Krasnikov, Dmitry V.
Yulin, Alexei
Zhukov, Alexey
Nasibulin, Albert G.
Scheblykin, Ivan
Pushkarev, Anatoly
Zenkevich, Andrei
Bisquert, Juan
Marunchenko, Alexandr
contents The transition to smart wearable and flexible optoelectronic devices communicating with each other and performing neuromorphic computing at the edge is a big goal in next-generation optoelectronics. These devices should perform their regular tasks supported by energy-efficient in-memory calculations. Here, we study the response of the CsPbBr$_3$ halide-perovskite single crystal fabricated on the flexible polymer substrate and integrated with the single-walled carbon nanotube thin film electrodes in a lateral geometry. We show both photodetection functions combined with the synaptic functionality in our device under the application of hybrid optoelectrical stimuli. Furthermore, we demonstrate that our device exhibits frequency-dependent bidirectional modification of synaptic weight with a sliding threshold similar to biologically plausible Bienenstock-Cooper-Munro learning. The demonstrated optoelectronic synaptic behavior in halide-perovskite single-crystals opens the opportunity for the development of hybrid organic-inorganic artificial visual systems.
format Preprint
id arxiv_https___arxiv_org_abs_2312_09314
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Biorealistic Response in Optoelectrically-Driven Flexible Halide-Perovskite Single-Crystal Memristors
Matchenya, Ivan
Khanas, Anton
Podgornyi, Roman
Shirkin, Daniil
Ekgardt, Alexey
Sizykh, Nikita
Anoshkin, Sergey
Krasnikov, Dmitry V.
Yulin, Alexei
Zhukov, Alexey
Nasibulin, Albert G.
Scheblykin, Ivan
Pushkarev, Anatoly
Zenkevich, Andrei
Bisquert, Juan
Marunchenko, Alexandr
Materials Science
Applied Physics
Optics
The transition to smart wearable and flexible optoelectronic devices communicating with each other and performing neuromorphic computing at the edge is a big goal in next-generation optoelectronics. These devices should perform their regular tasks supported by energy-efficient in-memory calculations. Here, we study the response of the CsPbBr$_3$ halide-perovskite single crystal fabricated on the flexible polymer substrate and integrated with the single-walled carbon nanotube thin film electrodes in a lateral geometry. We show both photodetection functions combined with the synaptic functionality in our device under the application of hybrid optoelectrical stimuli. Furthermore, we demonstrate that our device exhibits frequency-dependent bidirectional modification of synaptic weight with a sliding threshold similar to biologically plausible Bienenstock-Cooper-Munro learning. The demonstrated optoelectronic synaptic behavior in halide-perovskite single-crystals opens the opportunity for the development of hybrid organic-inorganic artificial visual systems.
title Biorealistic Response in Optoelectrically-Driven Flexible Halide-Perovskite Single-Crystal Memristors
topic Materials Science
Applied Physics
Optics
url https://arxiv.org/abs/2312.09314