Signature of pressure-induced topological phase transition in ZrTe$_5$

Fuente: arXiv
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Autores principales: Kovács-Krausz, Zoltán, Nagy, Dániel, Márffy, Albin, Karpiak, Bogdan, Tajkov, Zoltán, Oroszlány, László, Koltai, János, Nemes-Incze, Péter, Dash, Saroj P., Makk, Péter, Csonka, Szabolcs, Tóvári, Endre
Formato: Preprint
Publicado: 2023
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author Kovács-Krausz, Zoltán
Nagy, Dániel
Márffy, Albin
Karpiak, Bogdan
Tajkov, Zoltán
Oroszlány, László
Koltai, János
Nemes-Incze, Péter
Dash, Saroj P.
Makk, Péter
Csonka, Szabolcs
Tóvári, Endre
author_facet Kovács-Krausz, Zoltán
Nagy, Dániel
Márffy, Albin
Karpiak, Bogdan
Tajkov, Zoltán
Oroszlány, László
Koltai, János
Nemes-Incze, Péter
Dash, Saroj P.
Makk, Péter
Csonka, Szabolcs
Tóvári, Endre
contents The layered van der Waals material ZrTe$_5$ is known as a candidate topological insulator (TI), however its topological phase and the relation with other properties such as an apparent Dirac semimetallic state is still a subject of debate. We employ a semiclassical multicarrier transport (MCT) model to analyze the magnetotransport of ZrTe$_5$ nanodevices at hydrostatic pressures up to 2 GPa. The temperature dependence of the MCT results between 10 and 300 K is assessed in the context of thermal activation, and we obtain the positions of conduction and valence band edges in the vicinity of the chemical potential. We find evidence of the closing and re-opening of the band gap with increasing pressure, which is consistent with a phase transition from weak to strong TI. This matches expectations from ab initio band structure calculations, as well as previous observations that CVT-grown ZrTe$_5$ is a weak TI in ambient conditions.
format Preprint
id arxiv_https___arxiv_org_abs_2312_10223
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Signature of pressure-induced topological phase transition in ZrTe$_5$
Kovács-Krausz, Zoltán
Nagy, Dániel
Márffy, Albin
Karpiak, Bogdan
Tajkov, Zoltán
Oroszlány, László
Koltai, János
Nemes-Incze, Péter
Dash, Saroj P.
Makk, Péter
Csonka, Szabolcs
Tóvári, Endre
Mesoscale and Nanoscale Physics
Materials Science
The layered van der Waals material ZrTe$_5$ is known as a candidate topological insulator (TI), however its topological phase and the relation with other properties such as an apparent Dirac semimetallic state is still a subject of debate. We employ a semiclassical multicarrier transport (MCT) model to analyze the magnetotransport of ZrTe$_5$ nanodevices at hydrostatic pressures up to 2 GPa. The temperature dependence of the MCT results between 10 and 300 K is assessed in the context of thermal activation, and we obtain the positions of conduction and valence band edges in the vicinity of the chemical potential. We find evidence of the closing and re-opening of the band gap with increasing pressure, which is consistent with a phase transition from weak to strong TI. This matches expectations from ab initio band structure calculations, as well as previous observations that CVT-grown ZrTe$_5$ is a weak TI in ambient conditions.
title Signature of pressure-induced topological phase transition in ZrTe$_5$
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2312.10223