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Main Authors: Xie, Chendi, Smith, Adam D., Yan, Haoran, Chen, Wei-Chih, Wang, Yao
Format: Preprint
Published: 2023
Subjects:
Online Access:https://arxiv.org/abs/2312.12706
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author Xie, Chendi
Smith, Adam D.
Yan, Haoran
Chen, Wei-Chih
Wang, Yao
author_facet Xie, Chendi
Smith, Adam D.
Yan, Haoran
Chen, Wei-Chih
Wang, Yao
contents Metallic hydrogen and hydride materials stand as promising avenues to achieve room-temperature superconductivity. Characterized by their high phonon frequencies and moderate coupling strengths, several high-pressure hydrides were theoretically predicted to exhibit transition temperatures ($T_c$) exceeding 250\,K, a claim further substantiated by experimental evidence. In an effort to push $T_c$ beyond room temperature, we introduce a dynamical method that involves stimulating hydrides with mid-infrared lasers. Employing Floquet first-principles simulations, we observe that in a nonequilibrium state induced by light, both the electronic density of states and the coupling to high-energy phonons see notable enhancements. These simultaneous improvements collectively result in an estimated 20\%-30\% rise in $T_c$ in practical pump conditions. Our theoretical investigation, therefore, offers a novel strategy to potentially raise the $T_c$ of hydrides above room temperature.
format Preprint
id arxiv_https___arxiv_org_abs_2312_12706
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Dynamical Approach to Realize Room-Temperature Superconductivity in LaH$_{10}$
Xie, Chendi
Smith, Adam D.
Yan, Haoran
Chen, Wei-Chih
Wang, Yao
Superconductivity
Metallic hydrogen and hydride materials stand as promising avenues to achieve room-temperature superconductivity. Characterized by their high phonon frequencies and moderate coupling strengths, several high-pressure hydrides were theoretically predicted to exhibit transition temperatures ($T_c$) exceeding 250\,K, a claim further substantiated by experimental evidence. In an effort to push $T_c$ beyond room temperature, we introduce a dynamical method that involves stimulating hydrides with mid-infrared lasers. Employing Floquet first-principles simulations, we observe that in a nonequilibrium state induced by light, both the electronic density of states and the coupling to high-energy phonons see notable enhancements. These simultaneous improvements collectively result in an estimated 20\%-30\% rise in $T_c$ in practical pump conditions. Our theoretical investigation, therefore, offers a novel strategy to potentially raise the $T_c$ of hydrides above room temperature.
title Dynamical Approach to Realize Room-Temperature Superconductivity in LaH$_{10}$
topic Superconductivity
url https://arxiv.org/abs/2312.12706