Layer-dependent evolution of electronic structures and correlations in rhombohedral multilayer graphene
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arXiv
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2023
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| author | Zhang, Yang Zhou, Yue-Ying Zhang, Shihao Cai, Hao Tong, Ling-Hui Tian, Yuan Chen, Tongtong Tian, Qiwei Zhang, Chen Wang, Yiliu Zou, Xuming Liu, Xingqiang Hu, Yuanyuan Ren, Ya-Ning Zhang, Li Zhang, Lijie Wang, Wen-Xiao He, Lin Liao, Lei Qin, Zhihui Yin, Long-Jing |
| author_facet | Zhang, Yang Zhou, Yue-Ying Zhang, Shihao Cai, Hao Tong, Ling-Hui Tian, Yuan Chen, Tongtong Tian, Qiwei Zhang, Chen Wang, Yiliu Zou, Xuming Liu, Xingqiang Hu, Yuanyuan Ren, Ya-Ning Zhang, Li Zhang, Lijie Wang, Wen-Xiao He, Lin Liao, Lei Qin, Zhihui Yin, Long-Jing |
| contents | The recent discovery of superconductivity and magnetism in trilayer rhombohedral graphene (RG) establishes an ideal, untwisted platform to study strong correlation electronic phenomena. However, the correlated effects in multilayer RG have received limited attention, and, particularly, the evolution of the correlations with increasing layer number remains an unresolved question. Here, we show the observation of layer-dependent electronic structures and correlations, under surprising liquid nitrogen temperature, in RG multilayers from 3 to 9 layers by using scanning tunneling microscopy and spectroscopy. We explicitly determine layer-enhanced low-energy flat bands and interlayer coupling strengths. The former directly demonstrates the further flattening of low-energy bands in thicker RG, and the latter indicates the presence of varying interlayer interactions in RG multilayers. Moreover, we find significant splittings of the flat bands, ranging from ~50-80 meV, at 77 K when they are partially filled, indicating the emergence of interaction-induced strongly correlated states. Particularly, the strength of the correlated states is notably enhanced in thicker RG and reaches its maximum in the six-layer, validating directly theoretical predictions and establishing abundant new candidates for strongly correlated systems. Our results provide valuable insights into the layer dependence of the electronic properties in RG and demonstrate it as a suitable system for investigating robust and highly accessible correlated phases. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2312_13637 |
| institution | arXiv |
| publishDate | 2023 |
| record_format | arxiv |
| spellingShingle | Layer-dependent evolution of electronic structures and correlations in rhombohedral multilayer graphene Zhang, Yang Zhou, Yue-Ying Zhang, Shihao Cai, Hao Tong, Ling-Hui Tian, Yuan Chen, Tongtong Tian, Qiwei Zhang, Chen Wang, Yiliu Zou, Xuming Liu, Xingqiang Hu, Yuanyuan Ren, Ya-Ning Zhang, Li Zhang, Lijie Wang, Wen-Xiao He, Lin Liao, Lei Qin, Zhihui Yin, Long-Jing Mesoscale and Nanoscale Physics Strongly Correlated Electrons The recent discovery of superconductivity and magnetism in trilayer rhombohedral graphene (RG) establishes an ideal, untwisted platform to study strong correlation electronic phenomena. However, the correlated effects in multilayer RG have received limited attention, and, particularly, the evolution of the correlations with increasing layer number remains an unresolved question. Here, we show the observation of layer-dependent electronic structures and correlations, under surprising liquid nitrogen temperature, in RG multilayers from 3 to 9 layers by using scanning tunneling microscopy and spectroscopy. We explicitly determine layer-enhanced low-energy flat bands and interlayer coupling strengths. The former directly demonstrates the further flattening of low-energy bands in thicker RG, and the latter indicates the presence of varying interlayer interactions in RG multilayers. Moreover, we find significant splittings of the flat bands, ranging from ~50-80 meV, at 77 K when they are partially filled, indicating the emergence of interaction-induced strongly correlated states. Particularly, the strength of the correlated states is notably enhanced in thicker RG and reaches its maximum in the six-layer, validating directly theoretical predictions and establishing abundant new candidates for strongly correlated systems. Our results provide valuable insights into the layer dependence of the electronic properties in RG and demonstrate it as a suitable system for investigating robust and highly accessible correlated phases. |
| title | Layer-dependent evolution of electronic structures and correlations in rhombohedral multilayer graphene |
| topic | Mesoscale and Nanoscale Physics Strongly Correlated Electrons |
| url | https://arxiv.org/abs/2312.13637 |