Accelerating Plasmonic Hydrogen Sensors for Inert Gas Environments by Transformer-Based Deep Learning

Fuente: arXiv
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Auteurs principaux: Martvall, Viktor, Moberg, Henrik Klein, Theodoridis, Athanasios, Tomeček, David, Ekborg-Tanner, Pernilla, Nilsson, Sara, Volpe, Giovanni, Erhart, Paul, Langhammer, Christoph
Format: Preprint
Publié: 2023
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author Martvall, Viktor
Moberg, Henrik Klein
Theodoridis, Athanasios
Tomeček, David
Ekborg-Tanner, Pernilla
Nilsson, Sara
Volpe, Giovanni
Erhart, Paul
Langhammer, Christoph
author_facet Martvall, Viktor
Moberg, Henrik Klein
Theodoridis, Athanasios
Tomeček, David
Ekborg-Tanner, Pernilla
Nilsson, Sara
Volpe, Giovanni
Erhart, Paul
Langhammer, Christoph
contents The ability to rapidly detect hydrogen gas upon occurrence of a leak is critical for the safe large-scale implementation of hydrogen (energy) technologies. However, to date, no technically viable sensor solution exists that meets the corresponding response time targets set by stakeholders at technically relevant conditions. Here, we demonstrate how a tailored Long Short-term Transformer Ensemble Model for Accelerated Sensing (LEMAS) accelerates the response of a state-of-the-art optical plasmonic hydrogen sensor by up to a factor of 40 in an oxygen-free inert gas environment, by accurately predicting its response value to a hydrogen concentration change before it is physically reached by the sensor hardware. Furthermore, it eliminates the pressure dependence of the response intrinsic to metal hydride-based sensors, while leveraging their ability to operate in oxygen-starved environments that are proposed to be used for inert gas encapsulation systems of hydrogen installations. Moreover LEMAS provides a measure for the uncertainty of the predictions that is pivotal for safety-critical sensor applications. Our results thus advertise the use of deep learning for the acceleration of sensor response, also beyond the realm of plasmonic hydrogen detection.
format Preprint
id arxiv_https___arxiv_org_abs_2312_15372
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Accelerating Plasmonic Hydrogen Sensors for Inert Gas Environments by Transformer-Based Deep Learning
Martvall, Viktor
Moberg, Henrik Klein
Theodoridis, Athanasios
Tomeček, David
Ekborg-Tanner, Pernilla
Nilsson, Sara
Volpe, Giovanni
Erhart, Paul
Langhammer, Christoph
Computational Physics
Chemical Physics
Data Analysis, Statistics and Probability
The ability to rapidly detect hydrogen gas upon occurrence of a leak is critical for the safe large-scale implementation of hydrogen (energy) technologies. However, to date, no technically viable sensor solution exists that meets the corresponding response time targets set by stakeholders at technically relevant conditions. Here, we demonstrate how a tailored Long Short-term Transformer Ensemble Model for Accelerated Sensing (LEMAS) accelerates the response of a state-of-the-art optical plasmonic hydrogen sensor by up to a factor of 40 in an oxygen-free inert gas environment, by accurately predicting its response value to a hydrogen concentration change before it is physically reached by the sensor hardware. Furthermore, it eliminates the pressure dependence of the response intrinsic to metal hydride-based sensors, while leveraging their ability to operate in oxygen-starved environments that are proposed to be used for inert gas encapsulation systems of hydrogen installations. Moreover LEMAS provides a measure for the uncertainty of the predictions that is pivotal for safety-critical sensor applications. Our results thus advertise the use of deep learning for the acceleration of sensor response, also beyond the realm of plasmonic hydrogen detection.
title Accelerating Plasmonic Hydrogen Sensors for Inert Gas Environments by Transformer-Based Deep Learning
topic Computational Physics
Chemical Physics
Data Analysis, Statistics and Probability
url https://arxiv.org/abs/2312.15372