Heat conduction in magnetic insulators via hybridization of acoustic phonons and spin-flip excitations

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Auteurs principaux: Pocs, Christopher A., Leahy, Ian A., Xing, Jie, Choi, Eun Sang, Sefat, Athena S., Hermele, Michael, Lee, Minhyea
Format: Preprint
Publié: 2024
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author Pocs, Christopher A.
Leahy, Ian A.
Xing, Jie
Choi, Eun Sang
Sefat, Athena S.
Hermele, Michael
Lee, Minhyea
author_facet Pocs, Christopher A.
Leahy, Ian A.
Xing, Jie
Choi, Eun Sang
Sefat, Athena S.
Hermele, Michael
Lee, Minhyea
contents We present a comprehensive study on the longitudinal magneto-thermal transport in a paramagnetic effective spin-1/2 magnetic insulator CsYbSe$_2$, by introducing a minimal model requiring only Zeeman splitting and magnetoelastic coupling. We use it to argue that hybridized excitations -- formed from acoustic phonons and localized spin-flip-excitations across the Zeeman gap of the crystal electric field ground doublet -- are responsible for a non-monotonic field dependence of longitudinal thermal conductivity. Beyond highlighting a starring role for phonons, our results raise the prospect of universal magneto-thermal transport phenomena in paramagnetic insulators that originate from simple features shared across many systems.
format Preprint
id arxiv_https___arxiv_org_abs_2401_01407
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Heat conduction in magnetic insulators via hybridization of acoustic phonons and spin-flip excitations
Pocs, Christopher A.
Leahy, Ian A.
Xing, Jie
Choi, Eun Sang
Sefat, Athena S.
Hermele, Michael
Lee, Minhyea
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
We present a comprehensive study on the longitudinal magneto-thermal transport in a paramagnetic effective spin-1/2 magnetic insulator CsYbSe$_2$, by introducing a minimal model requiring only Zeeman splitting and magnetoelastic coupling. We use it to argue that hybridized excitations -- formed from acoustic phonons and localized spin-flip-excitations across the Zeeman gap of the crystal electric field ground doublet -- are responsible for a non-monotonic field dependence of longitudinal thermal conductivity. Beyond highlighting a starring role for phonons, our results raise the prospect of universal magneto-thermal transport phenomena in paramagnetic insulators that originate from simple features shared across many systems.
title Heat conduction in magnetic insulators via hybridization of acoustic phonons and spin-flip excitations
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2401.01407