Aggregation and charging of mineral cloud particles under high-energy irradiation

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Main Authors: Bach-Møller, Nanna, Helling, Christiane, Jørgensen, Uffe G., Enghoff, Martin B.
Format: Preprint
Published: 2024
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author Bach-Møller, Nanna
Helling, Christiane
Jørgensen, Uffe G.
Enghoff, Martin B.
author_facet Bach-Møller, Nanna
Helling, Christiane
Jørgensen, Uffe G.
Enghoff, Martin B.
contents It is known from Earth that ionizing high-energy radiation can lead to ion-induced nucleation of cloud condensation nuclei in the atmosphere. Since the amount of high-energy radiation can vary greatly based on the radiative environment of a host star, understanding the effect of high-energy radiation on cloud particles is critical to understand exoplanet atmospheres. This study aims to explore how high-energy radiation affects the aggregation and charging of mineral cloud particles. We present experiments conducted in an atmosphere chamber on mineral SiO$_2$ particles with diameters of 50 nm. The particles were exposed to gamma radiation in either low-humidity (RH $\approx$ 20%) or high-humidity (RH $>$ 50%) environments. The aggregation and charging state of the particles were studied with a Scanning Mobility Particle Sizer. We find that the single SiO$_2$ particles (N1) cluster to form larger aggregates (N2 - N4), and that this aggregation is inhibited by gamma radiation. We find that gamma radiation shifts the charging of the particles to become more negative, by increasing the charging state of negatively charged particles. Through an independent T-test we find that this increase is statistically significant within a 5% significance level for all aggregates in the high-humidity environment, and for all except the N1 particles in the low-humidity environment. For the positively charged particles the changes in charging state are not within the 5% significance level. We suggest that the overall effect of gamma radiation could favor the formation of a high number of small particles over a lower number of larger particles.
format Preprint
id arxiv_https___arxiv_org_abs_2401_03789
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Aggregation and charging of mineral cloud particles under high-energy irradiation
Bach-Møller, Nanna
Helling, Christiane
Jørgensen, Uffe G.
Enghoff, Martin B.
Earth and Planetary Astrophysics
Atmospheric and Oceanic Physics
It is known from Earth that ionizing high-energy radiation can lead to ion-induced nucleation of cloud condensation nuclei in the atmosphere. Since the amount of high-energy radiation can vary greatly based on the radiative environment of a host star, understanding the effect of high-energy radiation on cloud particles is critical to understand exoplanet atmospheres. This study aims to explore how high-energy radiation affects the aggregation and charging of mineral cloud particles. We present experiments conducted in an atmosphere chamber on mineral SiO$_2$ particles with diameters of 50 nm. The particles were exposed to gamma radiation in either low-humidity (RH $\approx$ 20%) or high-humidity (RH $>$ 50%) environments. The aggregation and charging state of the particles were studied with a Scanning Mobility Particle Sizer. We find that the single SiO$_2$ particles (N1) cluster to form larger aggregates (N2 - N4), and that this aggregation is inhibited by gamma radiation. We find that gamma radiation shifts the charging of the particles to become more negative, by increasing the charging state of negatively charged particles. Through an independent T-test we find that this increase is statistically significant within a 5% significance level for all aggregates in the high-humidity environment, and for all except the N1 particles in the low-humidity environment. For the positively charged particles the changes in charging state are not within the 5% significance level. We suggest that the overall effect of gamma radiation could favor the formation of a high number of small particles over a lower number of larger particles.
title Aggregation and charging of mineral cloud particles under high-energy irradiation
topic Earth and Planetary Astrophysics
Atmospheric and Oceanic Physics
url https://arxiv.org/abs/2401.03789