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Hauptverfasser: Mientjes, Mathijs G. C., Guan, Xin, Lueb, Pim J. H., Verheijen, Marcel A., Bakkers, Erik P. A. M.
Format: Preprint
Veröffentlicht: 2024
Schlagworte:
Online-Zugang:https://arxiv.org/abs/2401.04990
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author Mientjes, Mathijs G. C.
Guan, Xin
Lueb, Pim J. H.
Verheijen, Marcel A.
Bakkers, Erik P. A. M.
author_facet Mientjes, Mathijs G. C.
Guan, Xin
Lueb, Pim J. H.
Verheijen, Marcel A.
Bakkers, Erik P. A. M.
contents Topological crystalline insulators (TCIs) are interesting for their topological surface states, which hold great promise for scattering-free transport channels and fault-tolerant quantum computing. A promising TCI is SnTe. However, Sn-vacancies form in SnTe, causing a high hole density, hindering topological transport from the surface being measured. This issue could be relieved by using nanowires with a high surface-to-volume ratio. Furthermore, SnTe can be alloyed with Pb reducing the Sn-vacancies while maintaining its topological phase. Here we present the catalyst-free growth of monocrystalline PbSnTe in molecular beam epitaxy (MBE). By the addition of a pre-deposition stage before the growth, we have control over the nucleation phase and thereby increase the nanowire yield. This facilitates tuning the nanowire aspect ratio by a factor of four by varying the growth parameters. These results allow us to grow specific morphologies for future transport experiments to probe the topological surface states in a Pb1-xSnxTe-based platform.
format Preprint
id arxiv_https___arxiv_org_abs_2401_04990
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Catalyst-free MBE growth of PbSnTe nanowires with tunable aspect ratio
Mientjes, Mathijs G. C.
Guan, Xin
Lueb, Pim J. H.
Verheijen, Marcel A.
Bakkers, Erik P. A. M.
Materials Science
Topological crystalline insulators (TCIs) are interesting for their topological surface states, which hold great promise for scattering-free transport channels and fault-tolerant quantum computing. A promising TCI is SnTe. However, Sn-vacancies form in SnTe, causing a high hole density, hindering topological transport from the surface being measured. This issue could be relieved by using nanowires with a high surface-to-volume ratio. Furthermore, SnTe can be alloyed with Pb reducing the Sn-vacancies while maintaining its topological phase. Here we present the catalyst-free growth of monocrystalline PbSnTe in molecular beam epitaxy (MBE). By the addition of a pre-deposition stage before the growth, we have control over the nucleation phase and thereby increase the nanowire yield. This facilitates tuning the nanowire aspect ratio by a factor of four by varying the growth parameters. These results allow us to grow specific morphologies for future transport experiments to probe the topological surface states in a Pb1-xSnxTe-based platform.
title Catalyst-free MBE growth of PbSnTe nanowires with tunable aspect ratio
topic Materials Science
url https://arxiv.org/abs/2401.04990