Nematic quantum disordered state in FeSe

Fuente: arXiv
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Autori principali: Liu, Ruixian, Stone, Matthew B., Gao, Shang, Nakamura, Mitsutaka, Kamazawa, Kazuya, Krajewska, Aleksandra, Walker, Helen C., Cheng, Peng, Yu, Rong, Si, Qimiao, Dai, Pengcheng, Lu, Xingye
Natura: Preprint
Pubblicazione: 2024
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author Liu, Ruixian
Stone, Matthew B.
Gao, Shang
Nakamura, Mitsutaka
Kamazawa, Kazuya
Krajewska, Aleksandra
Walker, Helen C.
Cheng, Peng
Yu, Rong
Si, Qimiao
Dai, Pengcheng
Lu, Xingye
author_facet Liu, Ruixian
Stone, Matthew B.
Gao, Shang
Nakamura, Mitsutaka
Kamazawa, Kazuya
Krajewska, Aleksandra
Walker, Helen C.
Cheng, Peng
Yu, Rong
Si, Qimiao
Dai, Pengcheng
Lu, Xingye
contents The unusual quantum-disordered magnetic ground state intertwined with superconductivity and electronic nematicity in FeSe has been a research focus in iron-based superconductors. However, the intrinsic spin excitations across the entire Brillouin zone in detwinned FeSe, which forms the basis for a microscopic understanding of the magnetic state and superconductivity, remain to be determined. Here, we use inelastic neutron scattering to map out the spin excitations of FeSe dewtinned with a uniaxial-strain device. We find that the stripe spin excitations (Q=(1, 0)/(0, 1)) exhibit the $C_2$ symmetry up to $E\approx120$ meV, while the N{é}el spin excitations (Q=(1, 1)) retain their $C_4$ symmetry in the nematic state. The temperature dependence of the difference in the spin excitations at Q=(1, 0) and (0, 1) for temperatures above the structural phase transition unambiguously shows the establishment of the nematic quantum disordered state. The similarity of the Néel excitations in FeSe and NaFeAs suggests that the Néel excitations are driven by the enhanced electron correlations in the $3d_{xy}$ orbital. By determining the key features of the stripe excitations and fitting their dispersions using a Heisenberg Hamiltonian with biquadratic interaction ($J_1$-$K$-$J_2$), we establish a spin-interaction phase diagram and conclude that FeSe is close to a crossover region between the antiferroquadrupolar, Néel, and stripe ordering regimes. The results provide an experimental basis for establishing a microscopic theoretical model to describe the origin and intertwining of the emergent orders in iron-based superconductors.
format Preprint
id arxiv_https___arxiv_org_abs_2401_05092
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Nematic quantum disordered state in FeSe
Liu, Ruixian
Stone, Matthew B.
Gao, Shang
Nakamura, Mitsutaka
Kamazawa, Kazuya
Krajewska, Aleksandra
Walker, Helen C.
Cheng, Peng
Yu, Rong
Si, Qimiao
Dai, Pengcheng
Lu, Xingye
Superconductivity
Strongly Correlated Electrons
The unusual quantum-disordered magnetic ground state intertwined with superconductivity and electronic nematicity in FeSe has been a research focus in iron-based superconductors. However, the intrinsic spin excitations across the entire Brillouin zone in detwinned FeSe, which forms the basis for a microscopic understanding of the magnetic state and superconductivity, remain to be determined. Here, we use inelastic neutron scattering to map out the spin excitations of FeSe dewtinned with a uniaxial-strain device. We find that the stripe spin excitations (Q=(1, 0)/(0, 1)) exhibit the $C_2$ symmetry up to $E\approx120$ meV, while the N{é}el spin excitations (Q=(1, 1)) retain their $C_4$ symmetry in the nematic state. The temperature dependence of the difference in the spin excitations at Q=(1, 0) and (0, 1) for temperatures above the structural phase transition unambiguously shows the establishment of the nematic quantum disordered state. The similarity of the Néel excitations in FeSe and NaFeAs suggests that the Néel excitations are driven by the enhanced electron correlations in the $3d_{xy}$ orbital. By determining the key features of the stripe excitations and fitting their dispersions using a Heisenberg Hamiltonian with biquadratic interaction ($J_1$-$K$-$J_2$), we establish a spin-interaction phase diagram and conclude that FeSe is close to a crossover region between the antiferroquadrupolar, Néel, and stripe ordering regimes. The results provide an experimental basis for establishing a microscopic theoretical model to describe the origin and intertwining of the emergent orders in iron-based superconductors.
title Nematic quantum disordered state in FeSe
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2401.05092