Rydberg molecules bound by strong light fields

Fuente: arXiv
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Auteurs principaux: Hollerith, Simon, Walther, Valentin, Srakaew, Kritsana, Wei, David, Adler, Daniel, Agrawal, Suchita, Weckesser, Pascal, Bloch, Immanuel, Zeiher, Johannes
Format: Preprint
Publié: 2024
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author Hollerith, Simon
Walther, Valentin
Srakaew, Kritsana
Wei, David
Adler, Daniel
Agrawal, Suchita
Weckesser, Pascal
Bloch, Immanuel
Zeiher, Johannes
author_facet Hollerith, Simon
Walther, Valentin
Srakaew, Kritsana
Wei, David
Adler, Daniel
Agrawal, Suchita
Weckesser, Pascal
Bloch, Immanuel
Zeiher, Johannes
contents The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative mechanism and instead form bound states with the continuum of free motional states. This is enabled by the unique combination of extraordinarily slow vibrational motion in the molecular state and the optical coupling to a non-interacting continuum. Under conditions of strong coupling, we observe the emergence of distinct resonances and explain them within a Fano model. For atoms arranged on a lattice, we predict the strong continuum coupling to even stabilize molecules consisting of more than two atoms and find first signatures of these by observing atom loss correlations using a quantum gas microscope. Our results present an intriguing mechanism to control decoherence and bind multiatomic molecules using strong light-matter interactions.
format Preprint
id arxiv_https___arxiv_org_abs_2401_05129
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Rydberg molecules bound by strong light fields
Hollerith, Simon
Walther, Valentin
Srakaew, Kritsana
Wei, David
Adler, Daniel
Agrawal, Suchita
Weckesser, Pascal
Bloch, Immanuel
Zeiher, Johannes
Quantum Physics
Quantum Gases
Atomic Physics
The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative mechanism and instead form bound states with the continuum of free motional states. This is enabled by the unique combination of extraordinarily slow vibrational motion in the molecular state and the optical coupling to a non-interacting continuum. Under conditions of strong coupling, we observe the emergence of distinct resonances and explain them within a Fano model. For atoms arranged on a lattice, we predict the strong continuum coupling to even stabilize molecules consisting of more than two atoms and find first signatures of these by observing atom loss correlations using a quantum gas microscope. Our results present an intriguing mechanism to control decoherence and bind multiatomic molecules using strong light-matter interactions.
title Rydberg molecules bound by strong light fields
topic Quantum Physics
Quantum Gases
Atomic Physics
url https://arxiv.org/abs/2401.05129