Theoretical Design of Mono-Elemental Ferroelectricity with Tunable Spin Textures in Bilayer Tellurium

Fuente: arXiv
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Auteurs principaux: Zhu, Jiajun, Fu, Botao, Zhao, Heyun, Hu, Wanbiao
Format: Preprint
Publié: 2024
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author Zhu, Jiajun
Fu, Botao
Zhao, Heyun
Hu, Wanbiao
author_facet Zhu, Jiajun
Fu, Botao
Zhao, Heyun
Hu, Wanbiao
contents 2D Ferroelectricity with switchable electric polarization has drawn widespread attention in condensed matter physics due to its crucial applications in non-volatile memory and ferroelectric spin devices. Despite recent progress in 2D ferroelectric, achieving the mono-elemental ferroelectricity still remains a great challenge because most nonmetallic mono-elemental materials are stabilized in nonpolar crystal structures. In this work, we theoretically designed mono-elemental ferroelectricity with tunable and significant spin textures in bilayer tellurium (BL-Te). Comprehensive quantitative polarization calculations demonstrate that asymmetric stacking in BL-Te can generate out-of-plane (OOP) polarization with a magnitude of 0.78 pC/m. This polarization stems from distinguishing interlayer and intra-layer contributions. Moreover, these stacked BL-Te, characterized by significant spin-orbit coupling, serve as an ideal platform for investigating both conventional spin polarization and layer-dependent/hidden spin polarization through ferroelectric reversion. Our work not only broaden the category of 2D mono-elemental ferroelectric but also offer a new platform for multifunctional nanodevices.
format Preprint
id arxiv_https___arxiv_org_abs_2401_07752
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Theoretical Design of Mono-Elemental Ferroelectricity with Tunable Spin Textures in Bilayer Tellurium
Zhu, Jiajun
Fu, Botao
Zhao, Heyun
Hu, Wanbiao
Materials Science
Mesoscale and Nanoscale Physics
2D Ferroelectricity with switchable electric polarization has drawn widespread attention in condensed matter physics due to its crucial applications in non-volatile memory and ferroelectric spin devices. Despite recent progress in 2D ferroelectric, achieving the mono-elemental ferroelectricity still remains a great challenge because most nonmetallic mono-elemental materials are stabilized in nonpolar crystal structures. In this work, we theoretically designed mono-elemental ferroelectricity with tunable and significant spin textures in bilayer tellurium (BL-Te). Comprehensive quantitative polarization calculations demonstrate that asymmetric stacking in BL-Te can generate out-of-plane (OOP) polarization with a magnitude of 0.78 pC/m. This polarization stems from distinguishing interlayer and intra-layer contributions. Moreover, these stacked BL-Te, characterized by significant spin-orbit coupling, serve as an ideal platform for investigating both conventional spin polarization and layer-dependent/hidden spin polarization through ferroelectric reversion. Our work not only broaden the category of 2D mono-elemental ferroelectric but also offer a new platform for multifunctional nanodevices.
title Theoretical Design of Mono-Elemental Ferroelectricity with Tunable Spin Textures in Bilayer Tellurium
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2401.07752