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| Main Authors: | , , , |
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| Format: | Preprint |
| Published: |
2024
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| Subjects: | |
| Online Access: | https://arxiv.org/abs/2401.08029 |
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Table of Contents:
- We report on the CrFeTi$_2$O$_7$ (CFTO) system using a combination of x-ray diffraction, dc magnetization, ac susceptibility, specific heat and neutron diffraction measurements. CFTO is seen to crystallize in a monoclinic $P21/a$ symmetry. It shows a glassy freezing at $T{_f}$ ~ 22 K, characterized by the observation of bifurcation between ZFC and FC $χ$ (T) curves, frequency dispersion across $T{_f}$ in ac susceptibility, appearance of non-zero remanent magnetization and coercivity below $T{_f}$, very slow relaxation of iso-thermal remanent magnetization with time and a linear temperature dependence of magnetic contribution to specific heat $C{_m}$ below $T{_f}$. The microscopic neutron diffraction analysis of CFTO not only confirms the absence of long-range antiferromagnetic ordering but also exhibits diffuse scattering due to the presence of shortrange ordered antiferromagnetically correlated spin clusters.