The generative quantum eigensolver (GQE) and its application for ground state search

Fuente: arXiv
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Main Authors: Nakaji, Kouhei, Kristensen, Lasse Bjørn, Kemmoku, Ryota, Campos-Gonzalez-Angulo, Jorge A., Vakili, Mohammad Ghazi, Huang, Haozhe, Bagherimehrab, Mohsen, Gorgulla, Christoph, Wong, FuTe, McCaskey, Alex, Kim, Jin-Sung, Nguyen, Thien, Rao, Pooja, Gao, Qi, Sugawara, Michihiko, Yamamoto, Naoki, Aspuru-Guzik, Alán
Format: Preprint
Published: 2024
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author Nakaji, Kouhei
Kristensen, Lasse Bjørn
Kemmoku, Ryota
Campos-Gonzalez-Angulo, Jorge A.
Vakili, Mohammad Ghazi
Huang, Haozhe
Bagherimehrab, Mohsen
Gorgulla, Christoph
Wong, FuTe
McCaskey, Alex
Kim, Jin-Sung
Nguyen, Thien
Rao, Pooja
Gao, Qi
Sugawara, Michihiko
Yamamoto, Naoki
Aspuru-Guzik, Alán
author_facet Nakaji, Kouhei
Kristensen, Lasse Bjørn
Kemmoku, Ryota
Campos-Gonzalez-Angulo, Jorge A.
Vakili, Mohammad Ghazi
Huang, Haozhe
Bagherimehrab, Mohsen
Gorgulla, Christoph
Wong, FuTe
McCaskey, Alex
Kim, Jin-Sung
Nguyen, Thien
Rao, Pooja
Gao, Qi
Sugawara, Michihiko
Yamamoto, Naoki
Aspuru-Guzik, Alán
contents We introduce the generative quantum eigensolver (GQE), a new quantum computational framework that operates outside the variational quantum algorithm paradigm by applying classical generative models to quantum simulation. The GQE algorithm optimizes a classical generative model to produce quantum circuits with desired properties. Here, we develop a transformer-based implementation, which we name the generative pre-trained transformer-based (GPT) quantum eigensolver (GPT-QE). We show a proof-of-concept of training and pretraining of GPT-QE applied to electronic structure Hamiltonians, and demonstrate its ability illustrated by surpassing coupled cluster singles and doubles (CCSD) for the strong bond dissociation of the nitrogen molecule and approaching chemical accuracy. We also demonstrate the method on real quantum hardware.
format Preprint
id arxiv_https___arxiv_org_abs_2401_09253
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The generative quantum eigensolver (GQE) and its application for ground state search
Nakaji, Kouhei
Kristensen, Lasse Bjørn
Kemmoku, Ryota
Campos-Gonzalez-Angulo, Jorge A.
Vakili, Mohammad Ghazi
Huang, Haozhe
Bagherimehrab, Mohsen
Gorgulla, Christoph
Wong, FuTe
McCaskey, Alex
Kim, Jin-Sung
Nguyen, Thien
Rao, Pooja
Gao, Qi
Sugawara, Michihiko
Yamamoto, Naoki
Aspuru-Guzik, Alán
Quantum Physics
We introduce the generative quantum eigensolver (GQE), a new quantum computational framework that operates outside the variational quantum algorithm paradigm by applying classical generative models to quantum simulation. The GQE algorithm optimizes a classical generative model to produce quantum circuits with desired properties. Here, we develop a transformer-based implementation, which we name the generative pre-trained transformer-based (GPT) quantum eigensolver (GPT-QE). We show a proof-of-concept of training and pretraining of GPT-QE applied to electronic structure Hamiltonians, and demonstrate its ability illustrated by surpassing coupled cluster singles and doubles (CCSD) for the strong bond dissociation of the nitrogen molecule and approaching chemical accuracy. We also demonstrate the method on real quantum hardware.
title The generative quantum eigensolver (GQE) and its application for ground state search
topic Quantum Physics
url https://arxiv.org/abs/2401.09253