Laser cooling of a fermionic molecule

Fuente: arXiv
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Autores principales: Dai, Jinyu, Sun, Qi, Riley, Benjamin C., Mitra, Debayan, Zelevinsky, Tanya
Formato: Preprint
Publicado: 2024
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author Dai, Jinyu
Sun, Qi
Riley, Benjamin C.
Mitra, Debayan
Zelevinsky, Tanya
author_facet Dai, Jinyu
Sun, Qi
Riley, Benjamin C.
Mitra, Debayan
Zelevinsky, Tanya
contents Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold chemistry, quantum simulation, and precision measurements. Here we report direct laser cooling of a fermionic molecular isotopologue, calcium monodeuteride (CaD). With a nuclear spin I = 1, only 5 hyperfine states need to be addressed for rotational closure in optical cycling. These hyperfine states are unresolved for typical experimental linewidths. We present a method for efficiently producing alkaline-earth metal hydrides and deuterides. We demonstrate rotational closure and show magnetically assisted Sisyphus cooling in one dimension for a beam of CaD molecules. Our results indicate that the experimental complexity for laser cooling CaD is similar to that of calcium monohydride (CaH). Laser cooling of CaD is a promising first step for production of ultracold and trapped atomic deuterium.
format Preprint
id arxiv_https___arxiv_org_abs_2401_12145
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Laser cooling of a fermionic molecule
Dai, Jinyu
Sun, Qi
Riley, Benjamin C.
Mitra, Debayan
Zelevinsky, Tanya
Atomic Physics
Quantum Gases
Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold chemistry, quantum simulation, and precision measurements. Here we report direct laser cooling of a fermionic molecular isotopologue, calcium monodeuteride (CaD). With a nuclear spin I = 1, only 5 hyperfine states need to be addressed for rotational closure in optical cycling. These hyperfine states are unresolved for typical experimental linewidths. We present a method for efficiently producing alkaline-earth metal hydrides and deuterides. We demonstrate rotational closure and show magnetically assisted Sisyphus cooling in one dimension for a beam of CaD molecules. Our results indicate that the experimental complexity for laser cooling CaD is similar to that of calcium monohydride (CaH). Laser cooling of CaD is a promising first step for production of ultracold and trapped atomic deuterium.
title Laser cooling of a fermionic molecule
topic Atomic Physics
Quantum Gases
url https://arxiv.org/abs/2401.12145