Dynamical Chiral Nernst Effect in Twisted Van der Waals Few Layers

Fuente: arXiv
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Main Authors: Li, Juncheng, Zhai, Dawei, Xiao, Cong, Yao, Wang
Format: Preprint
Published: 2024
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author Li, Juncheng
Zhai, Dawei
Xiao, Cong
Yao, Wang
author_facet Li, Juncheng
Zhai, Dawei
Xiao, Cong
Yao, Wang
contents The Nernst effect is a fundamental thermoelectric conversion phenomenon that was deemed to be possible only in systems with magnetic field or magnetization. In this work, we propose a novel dynamical chiral Nernst effect that can appear in two-dimensional van der Waals materials with chiral structural symmetry in the absence of any magnetic degree of freedom. This unconventional effect is triggered by time variation of an out-of-plane electric field, and has an intrinsic quantum geometric origin linked to not only the intralayer center-of-mass motion but also the interlayer coherence of electronic states. We demonstrate the effect in twisted homobilayer and homotrilayer transition metal dichalcogenides, where the strong twisted interlayer coupling leads to sizable intrinsic Nernst conductivities well within the experimental capacity. This work suggests a new route for electric control of thermoelectric conversion.
format Preprint
id arxiv_https___arxiv_org_abs_2401_13278
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Dynamical Chiral Nernst Effect in Twisted Van der Waals Few Layers
Li, Juncheng
Zhai, Dawei
Xiao, Cong
Yao, Wang
Mesoscale and Nanoscale Physics
Materials Science
The Nernst effect is a fundamental thermoelectric conversion phenomenon that was deemed to be possible only in systems with magnetic field or magnetization. In this work, we propose a novel dynamical chiral Nernst effect that can appear in two-dimensional van der Waals materials with chiral structural symmetry in the absence of any magnetic degree of freedom. This unconventional effect is triggered by time variation of an out-of-plane electric field, and has an intrinsic quantum geometric origin linked to not only the intralayer center-of-mass motion but also the interlayer coherence of electronic states. We demonstrate the effect in twisted homobilayer and homotrilayer transition metal dichalcogenides, where the strong twisted interlayer coupling leads to sizable intrinsic Nernst conductivities well within the experimental capacity. This work suggests a new route for electric control of thermoelectric conversion.
title Dynamical Chiral Nernst Effect in Twisted Van der Waals Few Layers
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2401.13278