Site-selective preparation and multi-state readout of molecules in optical tweezers

Fuente: arXiv
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Bibliographic Details
Main Authors: Picard, Lewis R. B., Patenotte, Gabriel E., Park, Annie J., Gebretsadkan, Samuel F., Ni, Kang-Kuen
Format: Preprint
Published: 2024
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author Picard, Lewis R. B.
Patenotte, Gabriel E.
Park, Annie J.
Gebretsadkan, Samuel F.
Ni, Kang-Kuen
author_facet Picard, Lewis R. B.
Patenotte, Gabriel E.
Park, Annie J.
Gebretsadkan, Samuel F.
Ni, Kang-Kuen
contents Polar molecules are a quantum resource with rich internal structure that can be coherently controlled. The structure, however, also makes the state preparation and measurement (SPAM) of molecules challenging. We advance the SPAM of individual molecules assembled from constituent atoms trapped in optical tweezer arrays. Sites without NaCs molecules are eliminated using high-fidelity Cs atom detection, increasing the peak molecule filling fraction of the array threefold. We site-selectively initialize the array in a rotational qubit subspace that is insensitive to differential AC Stark shifts from the optical tweezer. Lastly, we detect multiple rotational states per experimental cycle by imaging atoms after sequential state-selective dissociations. These demonstrations extend the SPAM capabilities of molecules for quantum information, simulation, and metrology.
format Preprint
id arxiv_https___arxiv_org_abs_2401_13659
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Site-selective preparation and multi-state readout of molecules in optical tweezers
Picard, Lewis R. B.
Patenotte, Gabriel E.
Park, Annie J.
Gebretsadkan, Samuel F.
Ni, Kang-Kuen
Atomic Physics
Quantum Physics
Polar molecules are a quantum resource with rich internal structure that can be coherently controlled. The structure, however, also makes the state preparation and measurement (SPAM) of molecules challenging. We advance the SPAM of individual molecules assembled from constituent atoms trapped in optical tweezer arrays. Sites without NaCs molecules are eliminated using high-fidelity Cs atom detection, increasing the peak molecule filling fraction of the array threefold. We site-selectively initialize the array in a rotational qubit subspace that is insensitive to differential AC Stark shifts from the optical tweezer. Lastly, we detect multiple rotational states per experimental cycle by imaging atoms after sequential state-selective dissociations. These demonstrations extend the SPAM capabilities of molecules for quantum information, simulation, and metrology.
title Site-selective preparation and multi-state readout of molecules in optical tweezers
topic Atomic Physics
Quantum Physics
url https://arxiv.org/abs/2401.13659