Double pulse all-optical coherent control of ultrafast spin-reorientation in antiferromagnetic rare-earth orthoferrite

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Main Authors: Khokhlov, N. E., Dolgikh, A. E., Ivanov, B. A., Kimel, A. V.
Format: Preprint
Published: 2024
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_version_ 1866929329467817984
author Khokhlov, N. E.
Dolgikh, A. E.
Ivanov, B. A.
Kimel, A. V.
author_facet Khokhlov, N. E.
Dolgikh, A. E.
Ivanov, B. A.
Kimel, A. V.
contents A pair of circularly polarized laser pulses of opposite helicities are shown to control the route of spin reorientation phase transition in rare-earth antiferromagnetic orthoferrite (Sm$_{0.55}$Tb$_{0.45}$)FeO$_3$. The route can be efficiently controlled by the delay between the pulses and the sample temperature. Simulations employing previously published models of \mbox{laser-induced} spin dynamics in orthoferrites failed to reproduce the experimental results. We suggest that the failure is due to neglected temperature dependence of the antiferromagnetic resonance damping in the material. Taking into account the experimentally deduced temperature dependence of the damping, we obtained good agreement between the simulations and the experiment.
format Preprint
id arxiv_https___arxiv_org_abs_2401_15009
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Double pulse all-optical coherent control of ultrafast spin-reorientation in antiferromagnetic rare-earth orthoferrite
Khokhlov, N. E.
Dolgikh, A. E.
Ivanov, B. A.
Kimel, A. V.
Strongly Correlated Electrons
Other Condensed Matter
A pair of circularly polarized laser pulses of opposite helicities are shown to control the route of spin reorientation phase transition in rare-earth antiferromagnetic orthoferrite (Sm$_{0.55}$Tb$_{0.45}$)FeO$_3$. The route can be efficiently controlled by the delay between the pulses and the sample temperature. Simulations employing previously published models of \mbox{laser-induced} spin dynamics in orthoferrites failed to reproduce the experimental results. We suggest that the failure is due to neglected temperature dependence of the antiferromagnetic resonance damping in the material. Taking into account the experimentally deduced temperature dependence of the damping, we obtained good agreement between the simulations and the experiment.
title Double pulse all-optical coherent control of ultrafast spin-reorientation in antiferromagnetic rare-earth orthoferrite
topic Strongly Correlated Electrons
Other Condensed Matter
url https://arxiv.org/abs/2401.15009