Superconductivity in freestanding infinite-layer nickelate membranes

Fuente: arXiv
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Autores principales: Yan, Shengjun, Mao, Wei, Sun, Wenjie, Li, Yueying, Sun, Haoying, Yang, Jiangfeng, Hao, Bo, Guo, Wei, Nian, Leyan, Gu, Zhengbin, Wang, Peng, Nie, Yuefeng
Formato: Preprint
Publicado: 2024
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author Yan, Shengjun
Mao, Wei
Sun, Wenjie
Li, Yueying
Sun, Haoying
Yang, Jiangfeng
Hao, Bo
Guo, Wei
Nian, Leyan
Gu, Zhengbin
Wang, Peng
Nie, Yuefeng
author_facet Yan, Shengjun
Mao, Wei
Sun, Wenjie
Li, Yueying
Sun, Haoying
Yang, Jiangfeng
Hao, Bo
Guo, Wei
Nian, Leyan
Gu, Zhengbin
Wang, Peng
Nie, Yuefeng
contents The observation of superconductivity in infinite-layer nickelates has attracted significant attention due to its potential as a new platform for exploring high $ \mathrm{\textit{T}}_{c} $ superconductivity. However, thus far, superconductivity has only been observed in epitaxial thin films, which limits the manipulation capabilities and modulation methods compared to two-dimensional exfoliated materials. Given the exceptionally giant strain tunability and stacking capability of freestanding membranes, separating superconducting nickelates from the as-grown substrate is a novel way to engineer the superconductivity and uncover the underlying physics. Herein, we report the synthesis of the superconducting freestanding $ \mathrm{La}_{0.8}\mathrm{Sr}_{0.2}\mathrm{Ni}\mathrm{O}_{2} $ membranes ($ \mathrm{\textit{T}}_{c}\mathrm{=}\mathrm{10.9}\;\mathrm{K} $), emphasizing the crucial roles of the interface engineering in the precursor phase film growth and the quick transfer process in achieving superconductivity. Our work offers a new versatile platform for investigating the superconductivity in nickelates, such as the pairing symmetry via constructing Josephson tunneling junctions and higher $ \mathrm{\textit{T}}_{c} $ values via high-pressure experiments.
format Preprint
id arxiv_https___arxiv_org_abs_2401_15980
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Superconductivity in freestanding infinite-layer nickelate membranes
Yan, Shengjun
Mao, Wei
Sun, Wenjie
Li, Yueying
Sun, Haoying
Yang, Jiangfeng
Hao, Bo
Guo, Wei
Nian, Leyan
Gu, Zhengbin
Wang, Peng
Nie, Yuefeng
Superconductivity
Materials Science
Strongly Correlated Electrons
The observation of superconductivity in infinite-layer nickelates has attracted significant attention due to its potential as a new platform for exploring high $ \mathrm{\textit{T}}_{c} $ superconductivity. However, thus far, superconductivity has only been observed in epitaxial thin films, which limits the manipulation capabilities and modulation methods compared to two-dimensional exfoliated materials. Given the exceptionally giant strain tunability and stacking capability of freestanding membranes, separating superconducting nickelates from the as-grown substrate is a novel way to engineer the superconductivity and uncover the underlying physics. Herein, we report the synthesis of the superconducting freestanding $ \mathrm{La}_{0.8}\mathrm{Sr}_{0.2}\mathrm{Ni}\mathrm{O}_{2} $ membranes ($ \mathrm{\textit{T}}_{c}\mathrm{=}\mathrm{10.9}\;\mathrm{K} $), emphasizing the crucial roles of the interface engineering in the precursor phase film growth and the quick transfer process in achieving superconductivity. Our work offers a new versatile platform for investigating the superconductivity in nickelates, such as the pairing symmetry via constructing Josephson tunneling junctions and higher $ \mathrm{\textit{T}}_{c} $ values via high-pressure experiments.
title Superconductivity in freestanding infinite-layer nickelate membranes
topic Superconductivity
Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2401.15980