Fluctuation-mediated spin-orbit torque enhancement in the noncollinear antiferromagnet Mn3Ni0.35Cu0.65N

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Main Authors: Bose, Arnab, Saunderson, Tom G., Shahee, Aga, Zhang, Lichuan, Hajiri, Tetsuya, Rajan, Adithya, Go, Dongwook, Asano, Hidefumi, Schwingenschlögl, Udo, Manchon, Aurelien, Mokrousov, Yuriy, Kläui, Mathias
Format: Preprint
Published: 2024
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author Bose, Arnab
Saunderson, Tom G.
Shahee, Aga
Zhang, Lichuan
Hajiri, Tetsuya
Rajan, Adithya
Go, Dongwook
Asano, Hidefumi
Schwingenschlögl, Udo
Manchon, Aurelien
Mokrousov, Yuriy
Kläui, Mathias
author_facet Bose, Arnab
Saunderson, Tom G.
Shahee, Aga
Zhang, Lichuan
Hajiri, Tetsuya
Rajan, Adithya
Go, Dongwook
Asano, Hidefumi
Schwingenschlögl, Udo
Manchon, Aurelien
Mokrousov, Yuriy
Kläui, Mathias
contents The role of spin fluctuations near magnetic phase transitions is crucial for generating various exotic phenomena, including anomalies in the extraordinary Hall effect, excess spin-current generation through the spin-Hall effect (SHE), and enhanced spin-pumping, amongst others. In this study, we experimentally investigate the temperature dependence of spin-orbit torques (SOTs) generated by Mn3Ni0.35Cu0.65N (MNCN), a member of the noncollinear antiferromagnetic family that exhibits unconventional magnetotransport properties. Our work uncovers a strong and nontrivial temperature dependence of SOTs, peaking near the Néel temperature of MNCN, which cannot be explained by conventional intrinsic and extrinsic scattering mechanisms of the SHE. Notably, we measure a maximum SOT efficiency of 30%, which is substantially larger than that of commonly studied nonmagnetic materials such as Pt. Theoretical calculations confirm a negligible SHE and a strong orbital Hall effect that can explain the observed SOTs. We propose a previously unidentified mechanism wherein fluctuating antiferromagnetic moments trigger the generation of substantial orbital currents near the Néel temperature due to the emergence of scalar spin chirality. Our findings present an approach for enhancing SOTs, which holds promise for magnetic memory applications by leveraging antiferromagnetic spin fluctuations to amplify both orbital and spin currents.
format Preprint
id arxiv_https___arxiv_org_abs_2401_16021
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Fluctuation-mediated spin-orbit torque enhancement in the noncollinear antiferromagnet Mn3Ni0.35Cu0.65N
Bose, Arnab
Saunderson, Tom G.
Shahee, Aga
Zhang, Lichuan
Hajiri, Tetsuya
Rajan, Adithya
Go, Dongwook
Asano, Hidefumi
Schwingenschlögl, Udo
Manchon, Aurelien
Mokrousov, Yuriy
Kläui, Mathias
Mesoscale and Nanoscale Physics
The role of spin fluctuations near magnetic phase transitions is crucial for generating various exotic phenomena, including anomalies in the extraordinary Hall effect, excess spin-current generation through the spin-Hall effect (SHE), and enhanced spin-pumping, amongst others. In this study, we experimentally investigate the temperature dependence of spin-orbit torques (SOTs) generated by Mn3Ni0.35Cu0.65N (MNCN), a member of the noncollinear antiferromagnetic family that exhibits unconventional magnetotransport properties. Our work uncovers a strong and nontrivial temperature dependence of SOTs, peaking near the Néel temperature of MNCN, which cannot be explained by conventional intrinsic and extrinsic scattering mechanisms of the SHE. Notably, we measure a maximum SOT efficiency of 30%, which is substantially larger than that of commonly studied nonmagnetic materials such as Pt. Theoretical calculations confirm a negligible SHE and a strong orbital Hall effect that can explain the observed SOTs. We propose a previously unidentified mechanism wherein fluctuating antiferromagnetic moments trigger the generation of substantial orbital currents near the Néel temperature due to the emergence of scalar spin chirality. Our findings present an approach for enhancing SOTs, which holds promise for magnetic memory applications by leveraging antiferromagnetic spin fluctuations to amplify both orbital and spin currents.
title Fluctuation-mediated spin-orbit torque enhancement in the noncollinear antiferromagnet Mn3Ni0.35Cu0.65N
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2401.16021