Molecular Pairing in Twisted Bilayer Graphene Superconductivity
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2024
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| author | Wang, Yi-Jie Zhou, Geng-Dong Peng, Shi-Yu Lian, Biao Song, Zhi-Da |
| author_facet | Wang, Yi-Jie Zhou, Geng-Dong Peng, Shi-Yu Lian, Biao Song, Zhi-Da |
| contents | We propose a theory for how the weak phonon-mediated interaction ($J_{\rm A}\!=\!1\!\sim\!4$meV) wins over the prohibitive Coulomb repulsion ($U\!=\!30\!\sim\!60$meV) and leads to a superconductor in magic-angle twisted bilayer graphene (MATBG). We find the pairing mechanism akin to that in the A$_3$C$_{60}$ family of molecular superconductors: Each AA stacking region of MATBG resembles a C$_{60}$ molecule, in that optical phonons can dynamically lift the degeneracy of the moiré orbitals, in analogy to the dynamical Jahn-Teller effect. Such induced $J_{\rm A}$ has the form of an inter-valley anti-Hund's coupling and is less suppressed than $U$ by the Kondo screening near a Mott insulator. Additionally, we also considered an intra-orbital Hund's coupling $J_{\rm H}$ that originates from the on-site repulsion of a carbon atom. Under a reasonable approximation of the realistic model, we prove that the renormalized local interaction between quasi-particles must have a pairing (negative) channel in a doped correlated insulator at $ν=\pm(2+δν)$, albeit the bare interaction is positive definite. The proof is non-perturbative and based on exact asymptotic behaviors of the vertex function imposed by Ward identities. Existence of an optimal $U$ for superconductivity is predicted. We also analyzed the pairing symmetry. In a large area of the parameter space of $J_{\rm A}$, $J_{\rm H}$, the ground state has a nematic $d$-wave singlet pairing, which, however, can lead to a $p$-wave-like nodal structure due to the Berry's phase on Fermi surfaces (or Euler obstruction). |
| format | Preprint |
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arxiv_https___arxiv_org_abs_2402_00869 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Molecular Pairing in Twisted Bilayer Graphene Superconductivity Wang, Yi-Jie Zhou, Geng-Dong Peng, Shi-Yu Lian, Biao Song, Zhi-Da Superconductivity Strongly Correlated Electrons We propose a theory for how the weak phonon-mediated interaction ($J_{\rm A}\!=\!1\!\sim\!4$meV) wins over the prohibitive Coulomb repulsion ($U\!=\!30\!\sim\!60$meV) and leads to a superconductor in magic-angle twisted bilayer graphene (MATBG). We find the pairing mechanism akin to that in the A$_3$C$_{60}$ family of molecular superconductors: Each AA stacking region of MATBG resembles a C$_{60}$ molecule, in that optical phonons can dynamically lift the degeneracy of the moiré orbitals, in analogy to the dynamical Jahn-Teller effect. Such induced $J_{\rm A}$ has the form of an inter-valley anti-Hund's coupling and is less suppressed than $U$ by the Kondo screening near a Mott insulator. Additionally, we also considered an intra-orbital Hund's coupling $J_{\rm H}$ that originates from the on-site repulsion of a carbon atom. Under a reasonable approximation of the realistic model, we prove that the renormalized local interaction between quasi-particles must have a pairing (negative) channel in a doped correlated insulator at $ν=\pm(2+δν)$, albeit the bare interaction is positive definite. The proof is non-perturbative and based on exact asymptotic behaviors of the vertex function imposed by Ward identities. Existence of an optimal $U$ for superconductivity is predicted. We also analyzed the pairing symmetry. In a large area of the parameter space of $J_{\rm A}$, $J_{\rm H}$, the ground state has a nematic $d$-wave singlet pairing, which, however, can lead to a $p$-wave-like nodal structure due to the Berry's phase on Fermi surfaces (or Euler obstruction). |
| title | Molecular Pairing in Twisted Bilayer Graphene Superconductivity |
| topic | Superconductivity Strongly Correlated Electrons |
| url | https://arxiv.org/abs/2402.00869 |