Symmetry-selective quasiparticle scattering and electric field tunability of the ZrSiS surface electronic structure

Fuente: arXiv
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Auteurs principaux: Lodge, Michael S., Marcellina, Elizabeth, Zhu, Ziming, Li, Xiao-Ping, Kaczorowski, Dariusz, Fuhrer, Michael S., Yang, Shengyuan A., Weber, Bent
Format: Preprint
Publié: 2024
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author Lodge, Michael S.
Marcellina, Elizabeth
Zhu, Ziming
Li, Xiao-Ping
Kaczorowski, Dariusz
Fuhrer, Michael S.
Yang, Shengyuan A.
Weber, Bent
author_facet Lodge, Michael S.
Marcellina, Elizabeth
Zhu, Ziming
Li, Xiao-Ping
Kaczorowski, Dariusz
Fuhrer, Michael S.
Yang, Shengyuan A.
Weber, Bent
contents 3D Dirac semimetals with square-net non-symmorphic symmetry, such as ternary ZrXY (X=Si, Ge; Y=S, Se, Te) compounds, have attracted significant attention owing to the presence of topological nodal lines, loops, or networks in their bulk. Orbital symmetry plays a profound role such materials as the different branches of the nodal dispersion can be distinguished by their distinct orbital symmetry eigenvalues. The presence of different eigenvalues suggests that scattering between states of different orbital symmetry may be strongly suppressed. Indeed, in ZrSiS, there has been no clear experimental evidence of quasiparticle scattering between states of different symmetry eigenvalue has been reported at small wave vector $q$. Here we show, using quasiparticle interference (QPI), that atomic step-edges in the ZrSiS surface facilitate quasiparticle scattering between states of different symmetry eigenvalues. This symmetry eigenvalue mixing quasiparticle scattering is the first to be reported for ZrSiS and contrasts quasiparticle scattering with no mixing of symmetry eigenvalues, where the latter occurs with scatterers preserving the glide mirror symmetry of the crystal lattice, e.g., native point defects in ZrSiS. Finally, we show that the electronic structure of the ZrSiS surface, including its unique floating band surface state (FBSS), can be tuned by a vertical electric field locally applied by the tip of a scanning tunneling microscope (STM), enabling control of a spin-orbit induced avoided crossing near the Fermi level by as much as 300%.
format Preprint
id arxiv_https___arxiv_org_abs_2402_01177
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Symmetry-selective quasiparticle scattering and electric field tunability of the ZrSiS surface electronic structure
Lodge, Michael S.
Marcellina, Elizabeth
Zhu, Ziming
Li, Xiao-Ping
Kaczorowski, Dariusz
Fuhrer, Michael S.
Yang, Shengyuan A.
Weber, Bent
Mesoscale and Nanoscale Physics
Materials Science
3D Dirac semimetals with square-net non-symmorphic symmetry, such as ternary ZrXY (X=Si, Ge; Y=S, Se, Te) compounds, have attracted significant attention owing to the presence of topological nodal lines, loops, or networks in their bulk. Orbital symmetry plays a profound role such materials as the different branches of the nodal dispersion can be distinguished by their distinct orbital symmetry eigenvalues. The presence of different eigenvalues suggests that scattering between states of different orbital symmetry may be strongly suppressed. Indeed, in ZrSiS, there has been no clear experimental evidence of quasiparticle scattering between states of different symmetry eigenvalue has been reported at small wave vector $q$. Here we show, using quasiparticle interference (QPI), that atomic step-edges in the ZrSiS surface facilitate quasiparticle scattering between states of different symmetry eigenvalues. This symmetry eigenvalue mixing quasiparticle scattering is the first to be reported for ZrSiS and contrasts quasiparticle scattering with no mixing of symmetry eigenvalues, where the latter occurs with scatterers preserving the glide mirror symmetry of the crystal lattice, e.g., native point defects in ZrSiS. Finally, we show that the electronic structure of the ZrSiS surface, including its unique floating band surface state (FBSS), can be tuned by a vertical electric field locally applied by the tip of a scanning tunneling microscope (STM), enabling control of a spin-orbit induced avoided crossing near the Fermi level by as much as 300%.
title Symmetry-selective quasiparticle scattering and electric field tunability of the ZrSiS surface electronic structure
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2402.01177