Coexistence of Ferromagnetism and Antiferromagnetic Dimers in Topological Insulators

Fuente: arXiv
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Autori principali: Islam, Farhan, Schlagel, Deborah, Lee, Yongbin, Pakhira, Santanu, Pajerowski, Daniel M., Johnston, David C., Ke, Liqin, Vaknin, David, McQueeney, Robert J.
Natura: Preprint
Pubblicazione: 2024
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author Islam, Farhan
Schlagel, Deborah
Lee, Yongbin
Pakhira, Santanu
Pajerowski, Daniel M.
Johnston, David C.
Ke, Liqin
Vaknin, David
McQueeney, Robert J.
author_facet Islam, Farhan
Schlagel, Deborah
Lee, Yongbin
Pakhira, Santanu
Pajerowski, Daniel M.
Johnston, David C.
Ke, Liqin
Vaknin, David
McQueeney, Robert J.
contents The addition of magnetic impurities in topological insulators can drive ferromagnetic order that leads to novel quantum anomalous Hall transport well below the Curie temperature. The fragility of the quantized regime has been ascribed to the random nature of the magnetic moment distribution. Here, we refine this hypothesis by using inelastic neutron scattering and density-functional theory calculations to show that two antagonistic components define the magnetism in Mn-substituted SnTe, thereby limiting the effectiveness of dilute magnetic TIs. One component is strongly bound antiferromagnetic dimers that compete with ferromagnetic order. The other component consists of undimerized moments where ferromagnetic order develops via long-range interactions.
format Preprint
id arxiv_https___arxiv_org_abs_2402_01531
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Coexistence of Ferromagnetism and Antiferromagnetic Dimers in Topological Insulators
Islam, Farhan
Schlagel, Deborah
Lee, Yongbin
Pakhira, Santanu
Pajerowski, Daniel M.
Johnston, David C.
Ke, Liqin
Vaknin, David
McQueeney, Robert J.
Strongly Correlated Electrons
The addition of magnetic impurities in topological insulators can drive ferromagnetic order that leads to novel quantum anomalous Hall transport well below the Curie temperature. The fragility of the quantized regime has been ascribed to the random nature of the magnetic moment distribution. Here, we refine this hypothesis by using inelastic neutron scattering and density-functional theory calculations to show that two antagonistic components define the magnetism in Mn-substituted SnTe, thereby limiting the effectiveness of dilute magnetic TIs. One component is strongly bound antiferromagnetic dimers that compete with ferromagnetic order. The other component consists of undimerized moments where ferromagnetic order develops via long-range interactions.
title Coexistence of Ferromagnetism and Antiferromagnetic Dimers in Topological Insulators
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2402.01531