Optical absorption and photoluminescence of single layer boron nitride from a first principles cumulant approach

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Marini, Giovanni, Calandra, Matteo, Cudazzo, Pierluigi
Format: Preprint
Published: 2024
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866913371619590144
author Marini, Giovanni
Calandra, Matteo
Cudazzo, Pierluigi
author_facet Marini, Giovanni
Calandra, Matteo
Cudazzo, Pierluigi
contents The photoluminescence spectrum of a single-layer boron nitride remains elusive, marked by enigmatic satellites that hint at a significant but unidentified exciton-phonon coupling.Here, by employing a first principles approach based on the many-body cumulant expansion of the charge response, we calculate the optical absorption and photoluminescence of a single layer boron nitride. We identify the specific exciton-phonon scattering channels and unravel their impact on the optical absorption and photoluminescence spectra thereby providing an interpretation of the experimental features. Finally, we show that, even in a strongly polar material such as h-BN monolayer, the electron-hole interaction responsible for the excitonic effect results in the cancellation of the Frölich interaction at small phonon momenta. This effect is captured only if the invariance of the exciton-phonon matrix elements under unitary transformations in the Bloch functions manifold is preserved in the calculation.
format Preprint
id arxiv_https___arxiv_org_abs_2402_03826
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Optical absorption and photoluminescence of single layer boron nitride from a first principles cumulant approach
Marini, Giovanni
Calandra, Matteo
Cudazzo, Pierluigi
Materials Science
The photoluminescence spectrum of a single-layer boron nitride remains elusive, marked by enigmatic satellites that hint at a significant but unidentified exciton-phonon coupling.Here, by employing a first principles approach based on the many-body cumulant expansion of the charge response, we calculate the optical absorption and photoluminescence of a single layer boron nitride. We identify the specific exciton-phonon scattering channels and unravel their impact on the optical absorption and photoluminescence spectra thereby providing an interpretation of the experimental features. Finally, we show that, even in a strongly polar material such as h-BN monolayer, the electron-hole interaction responsible for the excitonic effect results in the cancellation of the Frölich interaction at small phonon momenta. This effect is captured only if the invariance of the exciton-phonon matrix elements under unitary transformations in the Bloch functions manifold is preserved in the calculation.
title Optical absorption and photoluminescence of single layer boron nitride from a first principles cumulant approach
topic Materials Science
url https://arxiv.org/abs/2402.03826