Probing magnetism in moiré heterostructures with quantum twisting microscopes

Fuente: arXiv
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Autori principali: Pichler, Fabian, Kadow, Wilhelm, Kuhlenkamp, Clemens, Knap, Michael
Natura: Preprint
Pubblicazione: 2024
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author Pichler, Fabian
Kadow, Wilhelm
Kuhlenkamp, Clemens
Knap, Michael
author_facet Pichler, Fabian
Kadow, Wilhelm
Kuhlenkamp, Clemens
Knap, Michael
contents Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum resolved spectrum of single-particle and collective excitations, can be used as a novel tool to distinguish between different types of magnetic order. To this end, we calculate the single-particle spectral function and the dynamical spin-structure factor for both a ferromagnetic and antiferromagnetic generalized Wigner crystal formed in fractionally filled moiré superlattices of transition metal dichalcogenide heterostructures. We demonstrate that magnetic order can be clearly identified in these response functions. Furthermore, we explore signatures of quantum phase transitions in the quantum twisting microscope response. We focus on the specific case of triangular moiré lattices at half filling, which have been proposed to host a topological phase transition between a chiral spin liquid and a 120 degree ordered state. Our work demonstrates the potential for quantum twisting microscopes to characterize quantum magnetism in moiré heterostructures.
format Preprint
id arxiv_https___arxiv_org_abs_2402_04311
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Probing magnetism in moiré heterostructures with quantum twisting microscopes
Pichler, Fabian
Kadow, Wilhelm
Kuhlenkamp, Clemens
Knap, Michael
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum resolved spectrum of single-particle and collective excitations, can be used as a novel tool to distinguish between different types of magnetic order. To this end, we calculate the single-particle spectral function and the dynamical spin-structure factor for both a ferromagnetic and antiferromagnetic generalized Wigner crystal formed in fractionally filled moiré superlattices of transition metal dichalcogenide heterostructures. We demonstrate that magnetic order can be clearly identified in these response functions. Furthermore, we explore signatures of quantum phase transitions in the quantum twisting microscope response. We focus on the specific case of triangular moiré lattices at half filling, which have been proposed to host a topological phase transition between a chiral spin liquid and a 120 degree ordered state. Our work demonstrates the potential for quantum twisting microscopes to characterize quantum magnetism in moiré heterostructures.
title Probing magnetism in moiré heterostructures with quantum twisting microscopes
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2402.04311