Nano-scale dynamics of hydrogen in VO$_{2}$ studied by $μ$SR

Fuente: arXiv
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Autori principali: Okabe, H., Hiraishi, M., Koda, A., Matsushita, Y., Ohsawa, T., Ohashi, N., Kadono, R.
Natura: Preprint
Pubblicazione: 2024
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author Okabe, H.
Hiraishi, M.
Koda, A.
Matsushita, Y.
Ohsawa, T.
Ohashi, N.
Kadono, R.
author_facet Okabe, H.
Hiraishi, M.
Koda, A.
Matsushita, Y.
Ohsawa, T.
Ohashi, N.
Kadono, R.
contents Hydrogen dynamics in the nanoscale region of VO$_{2}$ was investigated by muon spin rotation/relaxation ($μ$SR) technique. Positively charged muon acts as a light radioisotope of proton and can be used as a probe to explore the inside of materials from an atomic perspective. By analyzing the muon hopping rate and the spatial distribution of the $^{51}$V nuclear magnetic moments, we have identified two types of diffusion paths in VO$_{2}$ (via oxygen-muon bonds or defects) and the potential of a high diffusion coefficient in the 10$^{-10}$ cm$^{2}$/s range at ambient temperature. Our results provide valuable information for developing hydrogen-driven VO$_{2}$--related electronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2402_08894
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Nano-scale dynamics of hydrogen in VO$_{2}$ studied by $μ$SR
Okabe, H.
Hiraishi, M.
Koda, A.
Matsushita, Y.
Ohsawa, T.
Ohashi, N.
Kadono, R.
Materials Science
Hydrogen dynamics in the nanoscale region of VO$_{2}$ was investigated by muon spin rotation/relaxation ($μ$SR) technique. Positively charged muon acts as a light radioisotope of proton and can be used as a probe to explore the inside of materials from an atomic perspective. By analyzing the muon hopping rate and the spatial distribution of the $^{51}$V nuclear magnetic moments, we have identified two types of diffusion paths in VO$_{2}$ (via oxygen-muon bonds or defects) and the potential of a high diffusion coefficient in the 10$^{-10}$ cm$^{2}$/s range at ambient temperature. Our results provide valuable information for developing hydrogen-driven VO$_{2}$--related electronic devices.
title Nano-scale dynamics of hydrogen in VO$_{2}$ studied by $μ$SR
topic Materials Science
url https://arxiv.org/abs/2402.08894