Direct Exfoliation of Nanoribbons from Bulk van der Waals Crystals

Fuente: arXiv
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Autores principales: Saunders, Ashley P., Chen, Victoria, Wang, Jierong, Johnson, Amalya C., McKeown-Green, Amy S., Zeng, Helen J., Mac, T. Kien, Trinh, Tuan, Heinz, Tony F., Pop, Eric, Liu, Fang
Formato: Preprint
Publicado: 2024
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author Saunders, Ashley P.
Chen, Victoria
Wang, Jierong
Johnson, Amalya C.
McKeown-Green, Amy S.
Zeng, Helen J.
Mac, T. Kien
Trinh, Tuan
Heinz, Tony F.
Pop, Eric
Liu, Fang
author_facet Saunders, Ashley P.
Chen, Victoria
Wang, Jierong
Johnson, Amalya C.
McKeown-Green, Amy S.
Zeng, Helen J.
Mac, T. Kien
Trinh, Tuan
Heinz, Tony F.
Pop, Eric
Liu, Fang
contents Confinement of monolayers into quasi-one-dimensional atomically-thin nanoribbons could lead to novel quantum phenomena beyond those achieved in their bulk and monolayer counterparts. However, current experimental availability of nanoribbon species beyond graphene has been limited to bottom-up synthesis or top-down patterning. In this study, we introduce a versatile and direct lithography-free approach to exfoliate a variety of bulk van der Waals (vdW) crystals into nanoribbons. Akin to the Scotch tape exfoliation in producing monolayers, this technique provides convenient access to a wide range of nanoribbons derived from their corresponding bulk crystals, including MoS2, WS2, MoSe2, WSe2, MoTe2, WTe2, ReS2, and hBN. The nanoribbons are single-crystalline, parallel-aligned, flat, and have high aspect ratio. We demonstrated the electrical, magnetic, and optical properties from the confinement, strain, and edge configurations of these nanoribbons. This versatile preparation technique will pave the way for future experimental investigation and broad applications in optoelectronic, sensing, electronic and quantum devices.
format Preprint
id arxiv_https___arxiv_org_abs_2402_11392
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Direct Exfoliation of Nanoribbons from Bulk van der Waals Crystals
Saunders, Ashley P.
Chen, Victoria
Wang, Jierong
Johnson, Amalya C.
McKeown-Green, Amy S.
Zeng, Helen J.
Mac, T. Kien
Trinh, Tuan
Heinz, Tony F.
Pop, Eric
Liu, Fang
Materials Science
Confinement of monolayers into quasi-one-dimensional atomically-thin nanoribbons could lead to novel quantum phenomena beyond those achieved in their bulk and monolayer counterparts. However, current experimental availability of nanoribbon species beyond graphene has been limited to bottom-up synthesis or top-down patterning. In this study, we introduce a versatile and direct lithography-free approach to exfoliate a variety of bulk van der Waals (vdW) crystals into nanoribbons. Akin to the Scotch tape exfoliation in producing monolayers, this technique provides convenient access to a wide range of nanoribbons derived from their corresponding bulk crystals, including MoS2, WS2, MoSe2, WSe2, MoTe2, WTe2, ReS2, and hBN. The nanoribbons are single-crystalline, parallel-aligned, flat, and have high aspect ratio. We demonstrated the electrical, magnetic, and optical properties from the confinement, strain, and edge configurations of these nanoribbons. This versatile preparation technique will pave the way for future experimental investigation and broad applications in optoelectronic, sensing, electronic and quantum devices.
title Direct Exfoliation of Nanoribbons from Bulk van der Waals Crystals
topic Materials Science
url https://arxiv.org/abs/2402.11392