Time- and angle-resolved photoemission spectroscopy with wavelength-tunable pump and extreme ultraviolet probe enabled by twin synchronized amplifiers

Fuente: arXiv
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Autori principali: Suzuki, Takeshi, Zhong, Yigui, Liu, Kecheng, Kanai, Teruto, Itatani, Jiro, Okazaki, Kozo
Natura: Preprint
Pubblicazione: 2024
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author Suzuki, Takeshi
Zhong, Yigui
Liu, Kecheng
Kanai, Teruto
Itatani, Jiro
Okazaki, Kozo
author_facet Suzuki, Takeshi
Zhong, Yigui
Liu, Kecheng
Kanai, Teruto
Itatani, Jiro
Okazaki, Kozo
contents We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire oscillator. The typical probe energy is 21.7 eV, and the wavelength of the pump excitation is tuned between 2400 and 1200 nm by using the optical parametric amplifier. The total energy resolution of 133 meV is achieved, and the time resolution is dependent on the wavelength for the pump, typically better than 100 fs. This system enables the pump energy to be matched with a specific interband transition and to probe a wider energy-momentum space. We present the results for the prototypical materials of highly oriented pyrolytic graphite and Bi2Se3 to show the performance of our system.
format Preprint
id arxiv_https___arxiv_org_abs_2402_13460
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Time- and angle-resolved photoemission spectroscopy with wavelength-tunable pump and extreme ultraviolet probe enabled by twin synchronized amplifiers
Suzuki, Takeshi
Zhong, Yigui
Liu, Kecheng
Kanai, Teruto
Itatani, Jiro
Okazaki, Kozo
Materials Science
Strongly Correlated Electrons
We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire oscillator. The typical probe energy is 21.7 eV, and the wavelength of the pump excitation is tuned between 2400 and 1200 nm by using the optical parametric amplifier. The total energy resolution of 133 meV is achieved, and the time resolution is dependent on the wavelength for the pump, typically better than 100 fs. This system enables the pump energy to be matched with a specific interband transition and to probe a wider energy-momentum space. We present the results for the prototypical materials of highly oriented pyrolytic graphite and Bi2Se3 to show the performance of our system.
title Time- and angle-resolved photoemission spectroscopy with wavelength-tunable pump and extreme ultraviolet probe enabled by twin synchronized amplifiers
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2402.13460