Uniform large-area surface patterning achieved by metal dewetting for the top-down fabrication of GaN nanowire ensembles

Fuente: arXiv
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Main Authors: Kang, Jingxuan, Jose, Rose-Mary, Oliva, Miriam, Auzelle, Thomas, Ruiz, Mikel Gómez, Tahraoui, Abbes, Lähnemann, Jonas, Brandt, Oliver, Geelhaar, Lutz
Format: Preprint
Published: 2024
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author Kang, Jingxuan
Jose, Rose-Mary
Oliva, Miriam
Auzelle, Thomas
Ruiz, Mikel Gómez
Tahraoui, Abbes
Lähnemann, Jonas
Brandt, Oliver
Geelhaar, Lutz
author_facet Kang, Jingxuan
Jose, Rose-Mary
Oliva, Miriam
Auzelle, Thomas
Ruiz, Mikel Gómez
Tahraoui, Abbes
Lähnemann, Jonas
Brandt, Oliver
Geelhaar, Lutz
contents The dewetting of thin Pt films on different surfaces is investigated as a means to provide the patterning for the top-down fabrication of GaN nanowire ensembles. The transformation from a thin film to an ensemble of nanoislands upon annealing proceeds in good agreement with the void growth model. With increasing annealing duration, the size and shape uniformity of the nanoislands improves. This improvement speeds up for higher annealing temperature. After an optimum annealing duration, the size uniformity deteriorates due to the coalescence of neighboring islands. By changing the Pt film thickness, the nanoisland diameter and density can be quantitatively controlled in a way predicted by a simple thermodynamic model. We demonstrate the uniformity of the nanoisland ensembles for an area larger than 1 cm$^2$. GaN nanowires are fabricated by a sequence of dry and wet etching steps, and these nanowires inherit the diameters and density of the Pt nanoisland ensemble used as a mask. Our study achieves advancements in size uniformity and range of obtainable diameters compared to previous works. This simple, economical, and scalable approach to the top-down fabrication of nanowires is useful for applications requiring large and uniform nanowire ensembles with controllable dimensions.
format Preprint
id arxiv_https___arxiv_org_abs_2402_14375
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Uniform large-area surface patterning achieved by metal dewetting for the top-down fabrication of GaN nanowire ensembles
Kang, Jingxuan
Jose, Rose-Mary
Oliva, Miriam
Auzelle, Thomas
Ruiz, Mikel Gómez
Tahraoui, Abbes
Lähnemann, Jonas
Brandt, Oliver
Geelhaar, Lutz
Materials Science
Applied Physics
The dewetting of thin Pt films on different surfaces is investigated as a means to provide the patterning for the top-down fabrication of GaN nanowire ensembles. The transformation from a thin film to an ensemble of nanoislands upon annealing proceeds in good agreement with the void growth model. With increasing annealing duration, the size and shape uniformity of the nanoislands improves. This improvement speeds up for higher annealing temperature. After an optimum annealing duration, the size uniformity deteriorates due to the coalescence of neighboring islands. By changing the Pt film thickness, the nanoisland diameter and density can be quantitatively controlled in a way predicted by a simple thermodynamic model. We demonstrate the uniformity of the nanoisland ensembles for an area larger than 1 cm$^2$. GaN nanowires are fabricated by a sequence of dry and wet etching steps, and these nanowires inherit the diameters and density of the Pt nanoisland ensemble used as a mask. Our study achieves advancements in size uniformity and range of obtainable diameters compared to previous works. This simple, economical, and scalable approach to the top-down fabrication of nanowires is useful for applications requiring large and uniform nanowire ensembles with controllable dimensions.
title Uniform large-area surface patterning achieved by metal dewetting for the top-down fabrication of GaN nanowire ensembles
topic Materials Science
Applied Physics
url https://arxiv.org/abs/2402.14375