Radiative recombination rate suppressed in a quantum photocell with three electron donors

Fuente: arXiv
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Autores principales: Chen, Jing-Yi, Zhao, Shun-Cai
Formato: Preprint
Publicado: 2024
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author Chen, Jing-Yi
Zhao, Shun-Cai
author_facet Chen, Jing-Yi
Zhao, Shun-Cai
contents The radiative recombination of electron-hole pairs represents a great challenge to the photon-to-charge efficiency in photocell. In this paper, we visit the radiative recombination rate (RRR) in a quantum photocell with or without three dipole-dipole coupled electron donors. The results show that different gaps play the same roles while the ambient temperatures play different roles in the suppressed RRR with or without three dipole-dipole coupled electron donors. What's more, the dipole-dipole coupling strength J can greatly inhibit the RRRs with three dipole-dipole coupled electron donors, which indicates the quantum coherence generated by three coupled donors is an efficient approach to suppress RRR, and it is different from the quantum coherence mentioned by Marlan O. Scully [PRL 104, 207701 (2010)]. This presented scheme may propose some regulating strategies for efficient conversion efficiency via the suppressed RRR.
format Preprint
id arxiv_https___arxiv_org_abs_2402_15024
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Radiative recombination rate suppressed in a quantum photocell with three electron donors
Chen, Jing-Yi
Zhao, Shun-Cai
Mesoscale and Nanoscale Physics
Quantum Physics
The radiative recombination of electron-hole pairs represents a great challenge to the photon-to-charge efficiency in photocell. In this paper, we visit the radiative recombination rate (RRR) in a quantum photocell with or without three dipole-dipole coupled electron donors. The results show that different gaps play the same roles while the ambient temperatures play different roles in the suppressed RRR with or without three dipole-dipole coupled electron donors. What's more, the dipole-dipole coupling strength J can greatly inhibit the RRRs with three dipole-dipole coupled electron donors, which indicates the quantum coherence generated by three coupled donors is an efficient approach to suppress RRR, and it is different from the quantum coherence mentioned by Marlan O. Scully [PRL 104, 207701 (2010)]. This presented scheme may propose some regulating strategies for efficient conversion efficiency via the suppressed RRR.
title Radiative recombination rate suppressed in a quantum photocell with three electron donors
topic Mesoscale and Nanoscale Physics
Quantum Physics
url https://arxiv.org/abs/2402.15024