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Main Authors: Venkatesan, Balaji, Guan, Syu-You, Chang, Jen-Te, Chiu, Shiang-Bin, Yang, Po-Yuan, Su, Chih-Chuan, Chang, Tay-Rong, Raju, Kalaivanan, Sankar, Raman, Fongchaiya, Somboon, Chu, Ming-Wen, Chang, Chia-Seng, Chang, Guoqing, Lin, Hsin, Del Maestro, Adrian, Kao, Ying-Jer, Chuang, Tien-Ming
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2402.18893
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author Venkatesan, Balaji
Guan, Syu-You
Chang, Jen-Te
Chiu, Shiang-Bin
Yang, Po-Yuan
Su, Chih-Chuan
Chang, Tay-Rong
Raju, Kalaivanan
Sankar, Raman
Fongchaiya, Somboon
Chu, Ming-Wen
Chang, Chia-Seng
Chang, Guoqing
Lin, Hsin
Del Maestro, Adrian
Kao, Ying-Jer
Chuang, Tien-Ming
author_facet Venkatesan, Balaji
Guan, Syu-You
Chang, Jen-Te
Chiu, Shiang-Bin
Yang, Po-Yuan
Su, Chih-Chuan
Chang, Tay-Rong
Raju, Kalaivanan
Sankar, Raman
Fongchaiya, Somboon
Chu, Ming-Wen
Chang, Chia-Seng
Chang, Guoqing
Lin, Hsin
Del Maestro, Adrian
Kao, Ying-Jer
Chuang, Tien-Ming
contents Electronic liquid crystal (ELC) phases are spontaneous symmetry breaking states believed to arise from strong electron correlation in quantum materials such as cuprates and iron pnictides. Here, we report a direct observation of a smectic phase in a weakly correlated nonsymmorphic square-net semimetal GdSbxTe2-x. Incommensurate smectic charge modulation and intense local unidirectional nanostructure, which coexist with Dirac fermions across Fermi level, are visualized by using spectroscopic imaging - scanning tunneling microscopy. As materials with highly mobile carriers are mostly weakly correlated, the discovery of such an ELC phase are anomalous and raise questions on the origin of their emergence. Specifically, we demonstrate how chemical substitution generates these symmetry breaking phases before the system undergoes a charge density wave (CDW) - orthorhombic structural transition. Our results highlight the importance of impurities in realizing ELC phases and present a new material platform for exploring the interplay among quenched disorder, Dirac fermions and electron correlation.
format Preprint
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institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Direct Visualization of a Disorder Driven Electronic Smectic Phase in Nonsymmorphic Square-Net Semimetal GdSbTe
Venkatesan, Balaji
Guan, Syu-You
Chang, Jen-Te
Chiu, Shiang-Bin
Yang, Po-Yuan
Su, Chih-Chuan
Chang, Tay-Rong
Raju, Kalaivanan
Sankar, Raman
Fongchaiya, Somboon
Chu, Ming-Wen
Chang, Chia-Seng
Chang, Guoqing
Lin, Hsin
Del Maestro, Adrian
Kao, Ying-Jer
Chuang, Tien-Ming
Strongly Correlated Electrons
Materials Science
Electronic liquid crystal (ELC) phases are spontaneous symmetry breaking states believed to arise from strong electron correlation in quantum materials such as cuprates and iron pnictides. Here, we report a direct observation of a smectic phase in a weakly correlated nonsymmorphic square-net semimetal GdSbxTe2-x. Incommensurate smectic charge modulation and intense local unidirectional nanostructure, which coexist with Dirac fermions across Fermi level, are visualized by using spectroscopic imaging - scanning tunneling microscopy. As materials with highly mobile carriers are mostly weakly correlated, the discovery of such an ELC phase are anomalous and raise questions on the origin of their emergence. Specifically, we demonstrate how chemical substitution generates these symmetry breaking phases before the system undergoes a charge density wave (CDW) - orthorhombic structural transition. Our results highlight the importance of impurities in realizing ELC phases and present a new material platform for exploring the interplay among quenched disorder, Dirac fermions and electron correlation.
title Direct Visualization of a Disorder Driven Electronic Smectic Phase in Nonsymmorphic Square-Net Semimetal GdSbTe
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2402.18893