All epitaxial self-assembly of vertically-confined silicon color centers using ultra-low temperature epitaxy

Fuente: arXiv
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Autori principali: Aberl, Johannes, Navarrete, Enrique Prado, Karaman, Merve, Enriquez, Diego Haya, Wilflingseder, Christoph, Salomon, Andreas, Primetzhofer, Daniel, Schubert, Markus Andreas, Capellini, Giovanni, Fromherz, Thomas, Deák, Peter, Udvarhelyi, Péter, Song, Li, Gali, Ádám, Brehm, Moritz
Natura: Preprint
Pubblicazione: 2024
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author Aberl, Johannes
Navarrete, Enrique Prado
Karaman, Merve
Enriquez, Diego Haya
Wilflingseder, Christoph
Salomon, Andreas
Primetzhofer, Daniel
Schubert, Markus Andreas
Capellini, Giovanni
Fromherz, Thomas
Deák, Peter
Udvarhelyi, Péter
Song, Li
Gali, Ádám
Brehm, Moritz
author_facet Aberl, Johannes
Navarrete, Enrique Prado
Karaman, Merve
Enriquez, Diego Haya
Wilflingseder, Christoph
Salomon, Andreas
Primetzhofer, Daniel
Schubert, Markus Andreas
Capellini, Giovanni
Fromherz, Thomas
Deák, Peter
Udvarhelyi, Péter
Song, Li
Gali, Ádám
Brehm, Moritz
contents Silicon-based color-centers (SiCCs) have recently emerged as quantum-light sources that can be combined with telecom-range Si Photonics platforms. Unfortunately, using current SiCC fabrication, deterministic control over the vertical emitter position is impossible due to ion-implantation's stochastic nature. To overcome this bottleneck towards high-yield integration, we demonstrate a radically innovative creation method for various SiCCs, solely relying on epitaxial growth of Si and C-doped Si at atypically-low temperatures in a ultra-clean growth environment. These telecom emitters can be confined within sub-1nm thick layers embedded at arbitrary vertical positions within a highly crystalline Si matrix. Tuning growth conditions and doping, different SiCC types, e.g., W-centers, T-centers, G-centers, or derivatives like G'-centers can be created, which are particularly promising as Si-based single-photon sources and spin-photon interfaces. The zero-phonon emission from G'-centers can be conveniently tuned by the C-concentration, leading to a systematic wavelength shift and linewidth narrowing towards low emitter densities.
format Preprint
id arxiv_https___arxiv_org_abs_2402_19227
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle All epitaxial self-assembly of vertically-confined silicon color centers using ultra-low temperature epitaxy
Aberl, Johannes
Navarrete, Enrique Prado
Karaman, Merve
Enriquez, Diego Haya
Wilflingseder, Christoph
Salomon, Andreas
Primetzhofer, Daniel
Schubert, Markus Andreas
Capellini, Giovanni
Fromherz, Thomas
Deák, Peter
Udvarhelyi, Péter
Song, Li
Gali, Ádám
Brehm, Moritz
Mesoscale and Nanoscale Physics
Silicon-based color-centers (SiCCs) have recently emerged as quantum-light sources that can be combined with telecom-range Si Photonics platforms. Unfortunately, using current SiCC fabrication, deterministic control over the vertical emitter position is impossible due to ion-implantation's stochastic nature. To overcome this bottleneck towards high-yield integration, we demonstrate a radically innovative creation method for various SiCCs, solely relying on epitaxial growth of Si and C-doped Si at atypically-low temperatures in a ultra-clean growth environment. These telecom emitters can be confined within sub-1nm thick layers embedded at arbitrary vertical positions within a highly crystalline Si matrix. Tuning growth conditions and doping, different SiCC types, e.g., W-centers, T-centers, G-centers, or derivatives like G'-centers can be created, which are particularly promising as Si-based single-photon sources and spin-photon interfaces. The zero-phonon emission from G'-centers can be conveniently tuned by the C-concentration, leading to a systematic wavelength shift and linewidth narrowing towards low emitter densities.
title All epitaxial self-assembly of vertically-confined silicon color centers using ultra-low temperature epitaxy
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2402.19227