Controllable suppression of the unconventional superconductivity in bulk and thin-film Sr$_{2}$RuO$_{4}$ via high-energy electron irradiation

Fuente: arXiv
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Main Authors: Ruf, Jacob P., Noad, Hilary M. L., Grasset, Romain, Miao, Ludi, Zhakina, Elina, McGuinness, Philippa H., Nair, Hari P., Schreiber, Nathaniel J., Kikugawa, Naoki, Sokolov, Dmitry, Konczykowski, Marcin, Schlom, Darrell G., Shen, Kyle M., Mackenzie, Andrew P.
Format: Preprint
Published: 2024
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author Ruf, Jacob P.
Noad, Hilary M. L.
Grasset, Romain
Miao, Ludi
Zhakina, Elina
McGuinness, Philippa H.
Nair, Hari P.
Schreiber, Nathaniel J.
Kikugawa, Naoki
Sokolov, Dmitry
Konczykowski, Marcin
Schlom, Darrell G.
Shen, Kyle M.
Mackenzie, Andrew P.
author_facet Ruf, Jacob P.
Noad, Hilary M. L.
Grasset, Romain
Miao, Ludi
Zhakina, Elina
McGuinness, Philippa H.
Nair, Hari P.
Schreiber, Nathaniel J.
Kikugawa, Naoki
Sokolov, Dmitry
Konczykowski, Marcin
Schlom, Darrell G.
Shen, Kyle M.
Mackenzie, Andrew P.
contents In bulk Sr$_{2}$RuO$_{4}$, the strong sensitivity of the superconducting transition temperature $T_{\text{c}}$ to nonmagnetic impurities provides robust evidence for a superconducting order parameter that changes sign around the Fermi surface. In superconducting epitaxial thin-film Sr$_{2}$RuO$_{4}$, the relationship between $T_{\text{c}}$ and the residual resistivity $ρ_0$, which in bulk samples is taken to be a proxy for the low-temperature elastic scattering rate, is far less clear. Using high-energy electron irradiation to controllably introduce point disorder into bulk single-crystal and thin-film Sr$_{2}$RuO$_{4}$, we show that $T_{\text{c}}$ is suppressed in both systems at nearly identical rates. This suggests that part of $ρ_0$ in films comes from defects that do not contribute to superconducting pairbreaking, and establishes a quantitative link between the superconductivity of bulk and thin-film samples.
format Preprint
id arxiv_https___arxiv_org_abs_2402_19454
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Controllable suppression of the unconventional superconductivity in bulk and thin-film Sr$_{2}$RuO$_{4}$ via high-energy electron irradiation
Ruf, Jacob P.
Noad, Hilary M. L.
Grasset, Romain
Miao, Ludi
Zhakina, Elina
McGuinness, Philippa H.
Nair, Hari P.
Schreiber, Nathaniel J.
Kikugawa, Naoki
Sokolov, Dmitry
Konczykowski, Marcin
Schlom, Darrell G.
Shen, Kyle M.
Mackenzie, Andrew P.
Superconductivity
Materials Science
In bulk Sr$_{2}$RuO$_{4}$, the strong sensitivity of the superconducting transition temperature $T_{\text{c}}$ to nonmagnetic impurities provides robust evidence for a superconducting order parameter that changes sign around the Fermi surface. In superconducting epitaxial thin-film Sr$_{2}$RuO$_{4}$, the relationship between $T_{\text{c}}$ and the residual resistivity $ρ_0$, which in bulk samples is taken to be a proxy for the low-temperature elastic scattering rate, is far less clear. Using high-energy electron irradiation to controllably introduce point disorder into bulk single-crystal and thin-film Sr$_{2}$RuO$_{4}$, we show that $T_{\text{c}}$ is suppressed in both systems at nearly identical rates. This suggests that part of $ρ_0$ in films comes from defects that do not contribute to superconducting pairbreaking, and establishes a quantitative link between the superconductivity of bulk and thin-film samples.
title Controllable suppression of the unconventional superconductivity in bulk and thin-film Sr$_{2}$RuO$_{4}$ via high-energy electron irradiation
topic Superconductivity
Materials Science
url https://arxiv.org/abs/2402.19454