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Bibliographic Details
Main Authors: Sam, Jisvin, Mohakud, Sasmita, Wakabayashi, Katsunori, Dutta, Sudipta
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2403.03036
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Table of Contents:
  • Within first-principles calculations, we explore superconductivity in Ca-intercalated bilayer silicene compound, Si2CaSi2. This arises from the coupling of interlayer flower-like Γ-centered Fermi surface formed by the hybridization of Ca-3d and Si-3pz orbitals with low-energy out-of-plane vibrations enabled by silicene's buckling. The consequent large electron-phonon coupling, as evident from the Eliashberg spectral function leads to superconductivity below 5.4 K in this two-dimensional covalent system. Our results reveal the key control parameters to achieve superconductivity in experimentally synthesizable silicon-based thin materials that can find diverse applications.