Re-investigation of Moment Direction in a Kitaev Material $α$-RuCl$_{3}$

Fuente: arXiv
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Auteurs principaux: Kim, Subin, Horsley, Ezekiel, Nelson, Christie, Ruff, Jacob, Kim, Young-June
Format: Preprint
Publié: 2024
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author Kim, Subin
Horsley, Ezekiel
Nelson, Christie
Ruff, Jacob
Kim, Young-June
author_facet Kim, Subin
Horsley, Ezekiel
Nelson, Christie
Ruff, Jacob
Kim, Young-June
contents We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $α$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a high degree of structural twinning at low temperature, whereas the T$_{N}$=7.3K sample primarily comprises a single domain of R$\bar{3}$. Notwithstanding, both samples exhibit an identical zigzag magnetic structure, with magnetic moments pointing away from the honeycomb plane by $α=31(2)^{\circ}$. We argue that the identical ordered moment directions in these samples suggest that the intralayer magnetic Hamiltonian remains mostly unchanged regardless of T$_{N}$.
format Preprint
id arxiv_https___arxiv_org_abs_2403_04176
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Re-investigation of Moment Direction in a Kitaev Material $α$-RuCl$_{3}$
Kim, Subin
Horsley, Ezekiel
Nelson, Christie
Ruff, Jacob
Kim, Young-June
Strongly Correlated Electrons
We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $α$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a high degree of structural twinning at low temperature, whereas the T$_{N}$=7.3K sample primarily comprises a single domain of R$\bar{3}$. Notwithstanding, both samples exhibit an identical zigzag magnetic structure, with magnetic moments pointing away from the honeycomb plane by $α=31(2)^{\circ}$. We argue that the identical ordered moment directions in these samples suggest that the intralayer magnetic Hamiltonian remains mostly unchanged regardless of T$_{N}$.
title Re-investigation of Moment Direction in a Kitaev Material $α$-RuCl$_{3}$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2403.04176