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Main Authors: Ghorai, Gurupada, Ghosh, Kalyan, Patra, Abhilash, Samal, Prasanjit, Senapati, Kartik, Sahoo, Pratap K.
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2403.04426
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author Ghorai, Gurupada
Ghosh, Kalyan
Patra, Abhilash
Samal, Prasanjit
Senapati, Kartik
Sahoo, Pratap K.
author_facet Ghorai, Gurupada
Ghosh, Kalyan
Patra, Abhilash
Samal, Prasanjit
Senapati, Kartik
Sahoo, Pratap K.
contents Spin-phonon interaction plays an important role in 2D magnetic materials and motivates the development of next-generation spin- and charge-dependent microelectronic devices. Understanding the spin-phonon interaction by tuning the growth parameter of single crystal Cr$_2Te_3$, a robust quasi-2D room temperature magnetic material, is crucial for spintronic devices. The synthesis of single crystal 2D Cr$_2Te_3$ flakes on a Si substrate from co-deposited thin film by plasma annealing techniques is a significant achievement. The temperature dependence and polarization-resolved Raman spectroscopy with support of density functional theory classified lattice symmetry operations were used to identify the phonon modes to investigate the spin/electron-phonon interactions in Cr$_2Te_3$. The mean-field theory model in single crystal Cr$_2Te_3$ is employed to quantify the spin-phonon interaction and correlate with in-plane and out-of-plane magnetic behavior. The observation of a positive correlation between phonon mode frequency and spin-phonon interaction strength in single crystal Cr$_2Te_3$ can be a potential candidate for spintronic applications.
format Preprint
id arxiv_https___arxiv_org_abs_2403_04426
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Spin-Phonon interaction in quasi 2D- Cr$_2Te_3$
Ghorai, Gurupada
Ghosh, Kalyan
Patra, Abhilash
Samal, Prasanjit
Senapati, Kartik
Sahoo, Pratap K.
Materials Science
Spin-phonon interaction plays an important role in 2D magnetic materials and motivates the development of next-generation spin- and charge-dependent microelectronic devices. Understanding the spin-phonon interaction by tuning the growth parameter of single crystal Cr$_2Te_3$, a robust quasi-2D room temperature magnetic material, is crucial for spintronic devices. The synthesis of single crystal 2D Cr$_2Te_3$ flakes on a Si substrate from co-deposited thin film by plasma annealing techniques is a significant achievement. The temperature dependence and polarization-resolved Raman spectroscopy with support of density functional theory classified lattice symmetry operations were used to identify the phonon modes to investigate the spin/electron-phonon interactions in Cr$_2Te_3$. The mean-field theory model in single crystal Cr$_2Te_3$ is employed to quantify the spin-phonon interaction and correlate with in-plane and out-of-plane magnetic behavior. The observation of a positive correlation between phonon mode frequency and spin-phonon interaction strength in single crystal Cr$_2Te_3$ can be a potential candidate for spintronic applications.
title Spin-Phonon interaction in quasi 2D- Cr$_2Te_3$
topic Materials Science
url https://arxiv.org/abs/2403.04426