Enhancement of interlayer exciton emission in a TMDC heterostructure via a multi-resonant chirped microresonator up to room temperature
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| Main Authors: | , , , , , , , |
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| Format: | Preprint |
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2024
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| _version_ | 1866911792516562944 |
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| author | Palekar, Chirag C. Rosa, Barbara Heermeier, Niels Shih, Ching-Wen Limame, Imad Koulas-Simos, Aris Rahimi-Iman, Arash Reitzenstein, Stephan |
| author_facet | Palekar, Chirag C. Rosa, Barbara Heermeier, Niels Shih, Ching-Wen Limame, Imad Koulas-Simos, Aris Rahimi-Iman, Arash Reitzenstein, Stephan |
| contents | We report on multi-resonance chirped distributed Bragg reflector (DBR) microcavities. These systems are employed to investigate the light-mater interaction with both intra- and inter-layer excitons of transition metal dichalcogenide (TMDC) bilayer heterostructures. The chirped DBRs consisting of SiO2 and Si3N4 layers with gradually changing thickness exhibit a broad stopband with a width exceeding 600 nm. Importantly, and in contrast to conventional single-resonance microcavities, our structures provide multiple resonances across a broad spectral range, which can be matched to spectrally distinct resonances of the embedded TMDC heterostructures. We study cavity-coupled emission of both intra- and inter-layer excitons from an integrated WSe2/MoSe2 heterostructure in a chirped microcavity system. We observe an enhanced interlayer exciton emission with a Purcell factor of 6.67 +- 1.02 at 4 K. Additionally, we take advantage of cavity-enhanced emission of the interlayer exciton to investigate its temperature-dependent luminescence lifetime, which yields a value of 60 ps at room temperature. Our approach provides an intriguing platform for future studies of energetically distant and confined excitons in different semiconducting materials, which paves the way for various applications such as microlasers and single-photon sources by enabling precise control and manipulation of excitonic interactions utilizing multimode resonance light-matter interaction. |
| format | Preprint |
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arxiv_https___arxiv_org_abs_2403_06008 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Enhancement of interlayer exciton emission in a TMDC heterostructure via a multi-resonant chirped microresonator up to room temperature Palekar, Chirag C. Rosa, Barbara Heermeier, Niels Shih, Ching-Wen Limame, Imad Koulas-Simos, Aris Rahimi-Iman, Arash Reitzenstein, Stephan Mesoscale and Nanoscale Physics We report on multi-resonance chirped distributed Bragg reflector (DBR) microcavities. These systems are employed to investigate the light-mater interaction with both intra- and inter-layer excitons of transition metal dichalcogenide (TMDC) bilayer heterostructures. The chirped DBRs consisting of SiO2 and Si3N4 layers with gradually changing thickness exhibit a broad stopband with a width exceeding 600 nm. Importantly, and in contrast to conventional single-resonance microcavities, our structures provide multiple resonances across a broad spectral range, which can be matched to spectrally distinct resonances of the embedded TMDC heterostructures. We study cavity-coupled emission of both intra- and inter-layer excitons from an integrated WSe2/MoSe2 heterostructure in a chirped microcavity system. We observe an enhanced interlayer exciton emission with a Purcell factor of 6.67 +- 1.02 at 4 K. Additionally, we take advantage of cavity-enhanced emission of the interlayer exciton to investigate its temperature-dependent luminescence lifetime, which yields a value of 60 ps at room temperature. Our approach provides an intriguing platform for future studies of energetically distant and confined excitons in different semiconducting materials, which paves the way for various applications such as microlasers and single-photon sources by enabling precise control and manipulation of excitonic interactions utilizing multimode resonance light-matter interaction. |
| title | Enhancement of interlayer exciton emission in a TMDC heterostructure via a multi-resonant chirped microresonator up to room temperature |
| topic | Mesoscale and Nanoscale Physics |
| url | https://arxiv.org/abs/2403.06008 |