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Main Authors: Chang, Yue, Wan, Shuangai, Dong, Shichao, Qin, Jie
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2403.08300
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author Chang, Yue
Wan, Shuangai
Dong, Shichao
Qin, Jie
author_facet Chang, Yue
Wan, Shuangai
Dong, Shichao
Qin, Jie
contents Field-inhomogeneity-induced relaxation of atomic spins confined in vapor cells with depolarizing walls is studied. In contrast to nuclear spins, such as noble-gas spins, which experience minimal polarization loss at cell walls, atomic spins in uncoated cells undergo randomization at the boundaries. This distinct boundary condition results in a varied dependence of the relaxation rate on the field gradient. By solving the Bloch-Torrey equation under fully depolarizing boundary conditions, we illustrate that the relaxation rate induced by field inhomogeneity is more pronounced for spins with a smaller original relaxation rate (in the absence of the inhomogeneous field). We establish an upper limit for the relaxation rate through calculations in the perturbation regime. Moreover, we connect it to the spin-exchange-relaxation-free magnetometers, demonstrating that its linewidth is most sensitive to inhomogeneous fields along the magnetometer's sensitive axis. Our theoretical result agrees with the experimental data for cells subjected to small pump power. A deviation in high input-power scenarios arises from pump field attenuation, resulting in a non-uniformly distributed light shift that behaves like an inhomogeneous magnetic field.
format Preprint
id arxiv_https___arxiv_org_abs_2403_08300
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Spin relaxation in inhomogeneous magnetic fields with depolarizing boundaries
Chang, Yue
Wan, Shuangai
Dong, Shichao
Qin, Jie
Quantum Physics
Field-inhomogeneity-induced relaxation of atomic spins confined in vapor cells with depolarizing walls is studied. In contrast to nuclear spins, such as noble-gas spins, which experience minimal polarization loss at cell walls, atomic spins in uncoated cells undergo randomization at the boundaries. This distinct boundary condition results in a varied dependence of the relaxation rate on the field gradient. By solving the Bloch-Torrey equation under fully depolarizing boundary conditions, we illustrate that the relaxation rate induced by field inhomogeneity is more pronounced for spins with a smaller original relaxation rate (in the absence of the inhomogeneous field). We establish an upper limit for the relaxation rate through calculations in the perturbation regime. Moreover, we connect it to the spin-exchange-relaxation-free magnetometers, demonstrating that its linewidth is most sensitive to inhomogeneous fields along the magnetometer's sensitive axis. Our theoretical result agrees with the experimental data for cells subjected to small pump power. A deviation in high input-power scenarios arises from pump field attenuation, resulting in a non-uniformly distributed light shift that behaves like an inhomogeneous magnetic field.
title Spin relaxation in inhomogeneous magnetic fields with depolarizing boundaries
topic Quantum Physics
url https://arxiv.org/abs/2403.08300