Room temperature quantum emitters in van der Waals α-MoO3

Fuente: arXiv
Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: Lee, Jeonghan, Wang, Haiyuan, Park, Keun-Yeol, Huh, Soonsang, Kim, Donghan, Yu, Mihyang, Kim, Changyoung, Thygesen, Kristian Sommer, Lee, Jieun
Format: Preprint
Veröffentlicht: 2024
Schlagworte:
Online-Zugang:
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
_version_ 1866912186737098752
author Lee, Jeonghan
Wang, Haiyuan
Park, Keun-Yeol
Huh, Soonsang
Kim, Donghan
Yu, Mihyang
Kim, Changyoung
Thygesen, Kristian Sommer
Lee, Jieun
author_facet Lee, Jeonghan
Wang, Haiyuan
Park, Keun-Yeol
Huh, Soonsang
Kim, Donghan
Yu, Mihyang
Kim, Changyoung
Thygesen, Kristian Sommer
Lee, Jieun
contents Quantum emitters in solid-state materials are highly promising building blocks for quantum information processing and communication science. Recently, single-photon emission from van der Waals materials has been reported in transition metal dichalcogenides and hexagonal boron nitride, exhibiting the potential to realize photonic quantum technologies in two-dimensional materials. Here, we report the generation of room temperature single-photon emission from exfoliated and thermally annealed single crystals of van der Waals α-MoO3. The second-order correlation function measurement displays a clear photon antibunching, while the luminescence intensity exceeds 0.4 Mcts/s and remains stable under laser excitation. The theoretical calculation suggests that an oxygen vacancy defect is a possible candidate for the observed emitters. Together with photostability and brightness, quantum emitters in α-MoO3 provide a new avenue to realize photon-based quantum information science in van der Waals materials.
format Preprint
id arxiv_https___arxiv_org_abs_2403_09099
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Room temperature quantum emitters in van der Waals α-MoO3
Lee, Jeonghan
Wang, Haiyuan
Park, Keun-Yeol
Huh, Soonsang
Kim, Donghan
Yu, Mihyang
Kim, Changyoung
Thygesen, Kristian Sommer
Lee, Jieun
Materials Science
Optics
Quantum Physics
Quantum emitters in solid-state materials are highly promising building blocks for quantum information processing and communication science. Recently, single-photon emission from van der Waals materials has been reported in transition metal dichalcogenides and hexagonal boron nitride, exhibiting the potential to realize photonic quantum technologies in two-dimensional materials. Here, we report the generation of room temperature single-photon emission from exfoliated and thermally annealed single crystals of van der Waals α-MoO3. The second-order correlation function measurement displays a clear photon antibunching, while the luminescence intensity exceeds 0.4 Mcts/s and remains stable under laser excitation. The theoretical calculation suggests that an oxygen vacancy defect is a possible candidate for the observed emitters. Together with photostability and brightness, quantum emitters in α-MoO3 provide a new avenue to realize photon-based quantum information science in van der Waals materials.
title Room temperature quantum emitters in van der Waals α-MoO3
topic Materials Science
Optics
Quantum Physics
url https://arxiv.org/abs/2403.09099