Substrate, temperature and magnetic field dependence of electric polarisation in mixed-stacking tetralayer graphenes

Fuente: arXiv
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Autori principali: Sarsfield, Patrick Johansen, Garcia-Ruiz, Aitor, Fal'ko, Vladimir I.
Natura: Preprint
Pubblicazione: 2024
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author Sarsfield, Patrick Johansen
Garcia-Ruiz, Aitor
Fal'ko, Vladimir I.
author_facet Sarsfield, Patrick Johansen
Garcia-Ruiz, Aitor
Fal'ko, Vladimir I.
contents Polytypes of tetralayer graphene (TLG: Bernal, rhombohedral and mixed stacking) are crystalline structures with different symmetries. Among those, mixed-stacking tetralayers lack inversion symmetry, which allows for intrinsic spontaneous out-of-plane electrical polarisation, inverted in the mirror-image pair, ABCB and ABAC stackings. Here, we compare the intrinsic polarisation of such TLGs with the symmetry-breaking effect of a substrate, which can also generate out-of-plane electric dipole moments with different sizes in all four polytypes, including ABCB and ABAC twins. We analyse their temperature and magnetic field dependence, in view of understanding the origin of the recently measured Kelvin probe force microscopy maps of tetralayer flakes, and notice that the intrinsic contribution could be singled out based on magnetic field dependence of polarisation measured at low temperatures.
format Preprint
id arxiv_https___arxiv_org_abs_2403_09354
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Substrate, temperature and magnetic field dependence of electric polarisation in mixed-stacking tetralayer graphenes
Sarsfield, Patrick Johansen
Garcia-Ruiz, Aitor
Fal'ko, Vladimir I.
Mesoscale and Nanoscale Physics
Polytypes of tetralayer graphene (TLG: Bernal, rhombohedral and mixed stacking) are crystalline structures with different symmetries. Among those, mixed-stacking tetralayers lack inversion symmetry, which allows for intrinsic spontaneous out-of-plane electrical polarisation, inverted in the mirror-image pair, ABCB and ABAC stackings. Here, we compare the intrinsic polarisation of such TLGs with the symmetry-breaking effect of a substrate, which can also generate out-of-plane electric dipole moments with different sizes in all four polytypes, including ABCB and ABAC twins. We analyse their temperature and magnetic field dependence, in view of understanding the origin of the recently measured Kelvin probe force microscopy maps of tetralayer flakes, and notice that the intrinsic contribution could be singled out based on magnetic field dependence of polarisation measured at low temperatures.
title Substrate, temperature and magnetic field dependence of electric polarisation in mixed-stacking tetralayer graphenes
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2403.09354