Doppler-free three-photon spectroscopy on narrow-line optical transitions
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arXiv
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| Autores principales: | , , , |
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| Formato: | Preprint |
| Publicado: |
2024
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| _version_ | 1866912164523016192 |
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| author | Panelli, Guglielmo Burd, Shaun C. Porter, Erik J. Kasevich, Mark |
| author_facet | Panelli, Guglielmo Burd, Shaun C. Porter, Erik J. Kasevich, Mark |
| contents | We demonstrate coherent Doppler-free three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ optical clock transition and the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ intercombination transition in free-space thermal clouds of $^{88}$Sr atoms. By appropriate orientation of the wavevectors of three lasers incident on the atoms, the first-order Doppler shift can be eliminated for all velocity classes. Three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ transition enables high-contrast Ramsey spectroscopy with interrogation times comparable to the 21$μ$s natural lifetime using a single near-resonant laser source. Three-photon spectroscopy on the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ clock transition, using only laser frequencies nearly resonant with the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ and $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ transitions, enables a reduction in Doppler broadening by two orders of magnitude and a corresponding $\sim470$Hz linewidth without a confining potential. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2403_09814 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Doppler-free three-photon spectroscopy on narrow-line optical transitions Panelli, Guglielmo Burd, Shaun C. Porter, Erik J. Kasevich, Mark Atomic Physics Optics Quantum Physics We demonstrate coherent Doppler-free three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ optical clock transition and the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ intercombination transition in free-space thermal clouds of $^{88}$Sr atoms. By appropriate orientation of the wavevectors of three lasers incident on the atoms, the first-order Doppler shift can be eliminated for all velocity classes. Three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ transition enables high-contrast Ramsey spectroscopy with interrogation times comparable to the 21$μ$s natural lifetime using a single near-resonant laser source. Three-photon spectroscopy on the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ clock transition, using only laser frequencies nearly resonant with the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ and $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ transitions, enables a reduction in Doppler broadening by two orders of magnitude and a corresponding $\sim470$Hz linewidth without a confining potential. |
| title | Doppler-free three-photon spectroscopy on narrow-line optical transitions |
| topic | Atomic Physics Optics Quantum Physics |
| url | https://arxiv.org/abs/2403.09814 |