Quantum effects in the interaction of low-energy electrons with light

Fuente: arXiv
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Autores principales: Synanidis, Adamantios P., Gonçalves, P. A. D., Ropers, Claus, de Abajo, F. Javier García
Formato: Preprint
Publicado: 2024
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author Synanidis, Adamantios P.
Gonçalves, P. A. D.
Ropers, Claus
de Abajo, F. Javier García
author_facet Synanidis, Adamantios P.
Gonçalves, P. A. D.
Ropers, Claus
de Abajo, F. Javier García
contents The interaction between free electrons and nanoscale optical fields has emerged as a unique platform to investigate ultrafast processes in matter and explore fundamental quantum phenomena. In particular, optically modulated electrons are employed in ultrafast electron microscopy as noninvasive probes that push the limits of spatiotemporal and spectral resolution down to the picometer--attosecond--microelectronvolt range. Electron kinetic energies well above the involved photon energies are commonly employed, rendering the electron--light coupling efficiency low and, thus, only providing limited access to the wealth of quantum nonlinear phenomena underlying the dynamical response of nanostructures. Here, we theoretically investigate electron--light interactions when photons and electrons have comparable energies, revealing strong quantum and recoil effects that include a nonvanishing coupling of surface-scattered electrons to plane waves of light, inelastic electron backscattering from localized optical fields, and strong electron--light coupling under grazing electron diffraction by an illuminated crystal surface. Our results open new vistas in electron--light--matter interactions with promising applications in ultrafast electron microscopy.
format Preprint
id arxiv_https___arxiv_org_abs_2403_09896
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Quantum effects in the interaction of low-energy electrons with light
Synanidis, Adamantios P.
Gonçalves, P. A. D.
Ropers, Claus
de Abajo, F. Javier García
Mesoscale and Nanoscale Physics
The interaction between free electrons and nanoscale optical fields has emerged as a unique platform to investigate ultrafast processes in matter and explore fundamental quantum phenomena. In particular, optically modulated electrons are employed in ultrafast electron microscopy as noninvasive probes that push the limits of spatiotemporal and spectral resolution down to the picometer--attosecond--microelectronvolt range. Electron kinetic energies well above the involved photon energies are commonly employed, rendering the electron--light coupling efficiency low and, thus, only providing limited access to the wealth of quantum nonlinear phenomena underlying the dynamical response of nanostructures. Here, we theoretically investigate electron--light interactions when photons and electrons have comparable energies, revealing strong quantum and recoil effects that include a nonvanishing coupling of surface-scattered electrons to plane waves of light, inelastic electron backscattering from localized optical fields, and strong electron--light coupling under grazing electron diffraction by an illuminated crystal surface. Our results open new vistas in electron--light--matter interactions with promising applications in ultrafast electron microscopy.
title Quantum effects in the interaction of low-energy electrons with light
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2403.09896