Open quantum system simulation of time and frequency resolved spectroscopy
Fuente:
arXiv
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| Autore principale: | |
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| Natura: | Preprint |
| Pubblicazione: |
2024
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| Accesso online: | |
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| _version_ | 1866909976426971136 |
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| author | Kramer, Tobias |
| author_facet | Kramer, Tobias |
| contents | The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments and in photosynthetic complexes reaches a reaction center. The efficiency and time-scale depend not only on the excitonic couplings, but are also affected by the dissipation of energy to vibrational modes of the molecules. An open quantum system description provides a suitable tool to describe the involved processes and connects the decoherence and relaxation dynamics to measurements of the time-dependent polarization. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2403_10192 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Open quantum system simulation of time and frequency resolved spectroscopy Kramer, Tobias Quantum Physics Biological Physics The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments and in photosynthetic complexes reaches a reaction center. The efficiency and time-scale depend not only on the excitonic couplings, but are also affected by the dissipation of energy to vibrational modes of the molecules. An open quantum system description provides a suitable tool to describe the involved processes and connects the decoherence and relaxation dynamics to measurements of the time-dependent polarization. |
| title | Open quantum system simulation of time and frequency resolved spectroscopy |
| topic | Quantum Physics Biological Physics |
| url | https://arxiv.org/abs/2403.10192 |