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Main Authors: Liu, Fang, Skruszewicz, Slawomir, Späthe, Julian, Zhang, Yinyu, Hell, Sebastian, Ying, Bo, Paulus, Gerhard G., Kiss, Bálint, Murari, Krishna, Khalil, Malin, Cormier, Eric, Jiao, Li Guang, Fritzsche, Stephan, Kübel, Matthias
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2403.10473
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author Liu, Fang
Skruszewicz, Slawomir
Späthe, Julian
Zhang, Yinyu
Hell, Sebastian
Ying, Bo
Paulus, Gerhard G.
Kiss, Bálint
Murari, Krishna
Khalil, Malin
Cormier, Eric
Jiao, Li Guang
Fritzsche, Stephan
Kübel, Matthias
author_facet Liu, Fang
Skruszewicz, Slawomir
Späthe, Julian
Zhang, Yinyu
Hell, Sebastian
Ying, Bo
Paulus, Gerhard G.
Kiss, Bálint
Murari, Krishna
Khalil, Malin
Cormier, Eric
Jiao, Li Guang
Fritzsche, Stephan
Kübel, Matthias
contents Strong-field ionization can induce electron motion in both the continuum and the valence shell of the parent ion. Here, we explore their interplay by studying laser-induced electron diffraction (LIED) patterns arising from interaction with the potentials of two-hole states of the xenon cation. The quantitative rescattering theory is used to calculate the corresponding photoelectron momentum distributions, providing evidence that the spin-orbit dynamics could be detected by LIED. We identify the contribution of these time-evolving hole states to the angular distribution of the rescattered electrons, particularly noting a distinct change along the backward scattering angles. We benchmark numerical results with experiments using ultrabroad and femtosecond laser pulses centered at \SI{3100}{nm}.
format Preprint
id arxiv_https___arxiv_org_abs_2403_10473
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Exploring Valence Electron Dynamics of Xenon through Laser-Induced Electron Diffraction
Liu, Fang
Skruszewicz, Slawomir
Späthe, Julian
Zhang, Yinyu
Hell, Sebastian
Ying, Bo
Paulus, Gerhard G.
Kiss, Bálint
Murari, Krishna
Khalil, Malin
Cormier, Eric
Jiao, Li Guang
Fritzsche, Stephan
Kübel, Matthias
Atomic Physics
Strong-field ionization can induce electron motion in both the continuum and the valence shell of the parent ion. Here, we explore their interplay by studying laser-induced electron diffraction (LIED) patterns arising from interaction with the potentials of two-hole states of the xenon cation. The quantitative rescattering theory is used to calculate the corresponding photoelectron momentum distributions, providing evidence that the spin-orbit dynamics could be detected by LIED. We identify the contribution of these time-evolving hole states to the angular distribution of the rescattered electrons, particularly noting a distinct change along the backward scattering angles. We benchmark numerical results with experiments using ultrabroad and femtosecond laser pulses centered at \SI{3100}{nm}.
title Exploring Valence Electron Dynamics of Xenon through Laser-Induced Electron Diffraction
topic Atomic Physics
url https://arxiv.org/abs/2403.10473