The effect of Coulomb assisted hopping on STM signal: extended two site Hubbard model analysis

Fuente: arXiv
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Autor principal: Goldstein, Garry
Formato: Preprint
Publicado: 2024
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author Goldstein, Garry
author_facet Goldstein, Garry
contents In this work we study STM signal in the presence of Coulomb assisted hopping. We perform an extended two site Hubbard model analysis between the atom on the tip and the atom in the sample nearest to each other. We show that in the presence of Coulomb assisted hopping the STM signal depends on several spectral functions thereby complicating its interpretation. Furthermore in the broadband tip limit there are now three different competing rates for the total current (instead of one for the usual two site Hubbard model analysis used in the literature so far). We find an exact (within the Fermi golden rule - that is in the limit of weak coupling between tip and sample) expression for the current as a function of the bias voltage. As an example we apply our calculations to the case of free fermions with a uniform density of states. Even in this simple case there are non-trivial corrections - where the $dI/d\mathcal{V}$ (the rate of change of the current with respect to bias voltage) is not uniform as a two site (non-extended) Hubbard model analysis would predict. We also show that for realistic conditions the corrections predicted here are order one.
format Preprint
id arxiv_https___arxiv_org_abs_2403_11566
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The effect of Coulomb assisted hopping on STM signal: extended two site Hubbard model analysis
Goldstein, Garry
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Other Condensed Matter
In this work we study STM signal in the presence of Coulomb assisted hopping. We perform an extended two site Hubbard model analysis between the atom on the tip and the atom in the sample nearest to each other. We show that in the presence of Coulomb assisted hopping the STM signal depends on several spectral functions thereby complicating its interpretation. Furthermore in the broadband tip limit there are now three different competing rates for the total current (instead of one for the usual two site Hubbard model analysis used in the literature so far). We find an exact (within the Fermi golden rule - that is in the limit of weak coupling between tip and sample) expression for the current as a function of the bias voltage. As an example we apply our calculations to the case of free fermions with a uniform density of states. Even in this simple case there are non-trivial corrections - where the $dI/d\mathcal{V}$ (the rate of change of the current with respect to bias voltage) is not uniform as a two site (non-extended) Hubbard model analysis would predict. We also show that for realistic conditions the corrections predicted here are order one.
title The effect of Coulomb assisted hopping on STM signal: extended two site Hubbard model analysis
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Other Condensed Matter
url https://arxiv.org/abs/2403.11566