Size-dependent ferroelectric-to-paraelectric sliding transformations and antipolar-to-ferroelectric topological phase transitions in binary homobilayers

Fuente: arXiv
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Autores principales: Alejandro, Pacheco-Sanjuan, Pradeep, Kumar, Salvador, Barraza-Lopez
Formato: Preprint
Publicado: 2024
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author Alejandro, Pacheco-Sanjuan
Pradeep, Kumar
Salvador, Barraza-Lopez
author_facet Alejandro, Pacheco-Sanjuan
Pradeep, Kumar
Salvador, Barraza-Lopez
contents The recent discovery of ferroelectric behavior in few-layer materials, accompanied by the observation of antipolar domains in hexagonal boron nitride and transition metal dichalcogenide moiré bilayers, is paving the way for revolutionary advancements in the generation and manipulation of intrinsic electric dipoles through stacking. In addition, these cutting-edge quantum materials are reshaping our comprehension of phase transitions. Within the present study, we unveil a hitherto unreported size-dependent sliding behavior that marks a significant departure from conventional ferroelectrics. We also shed light on thermally induced spontaneous hyperlubric sliding within moiré bilayers, which can be used as a signal to distinguish topological phase transitions from an antipolar onto a ferroelectric bilayer. Our findings also suggest that the (topological) pinning of AA nodes in antipolar moiré homobilayers prevents the occurrence of an antipolar-to-paraelectric transformation.
format Preprint
id arxiv_https___arxiv_org_abs_2403_12175
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Size-dependent ferroelectric-to-paraelectric sliding transformations and antipolar-to-ferroelectric topological phase transitions in binary homobilayers
Alejandro, Pacheco-Sanjuan
Pradeep, Kumar
Salvador, Barraza-Lopez
Materials Science
Mesoscale and Nanoscale Physics
The recent discovery of ferroelectric behavior in few-layer materials, accompanied by the observation of antipolar domains in hexagonal boron nitride and transition metal dichalcogenide moiré bilayers, is paving the way for revolutionary advancements in the generation and manipulation of intrinsic electric dipoles through stacking. In addition, these cutting-edge quantum materials are reshaping our comprehension of phase transitions. Within the present study, we unveil a hitherto unreported size-dependent sliding behavior that marks a significant departure from conventional ferroelectrics. We also shed light on thermally induced spontaneous hyperlubric sliding within moiré bilayers, which can be used as a signal to distinguish topological phase transitions from an antipolar onto a ferroelectric bilayer. Our findings also suggest that the (topological) pinning of AA nodes in antipolar moiré homobilayers prevents the occurrence of an antipolar-to-paraelectric transformation.
title Size-dependent ferroelectric-to-paraelectric sliding transformations and antipolar-to-ferroelectric topological phase transitions in binary homobilayers
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2403.12175